Assessment and prediction of the impact of road transport on ambient concentrations of particulate matter PM10

Abstract The main challenge facing the air quality management authorities in most cities is meeting the air quality limits and objectives in areas where road traffic is high. The difficulty and uncertainties associated with the estimation and prediction of the road traffic contribution to the overall air quality levels is the major contributing factor. In this paper, particulate matter (PM10) data from 10 monitoring sites in London was investigated with a view to estimating and developing Artificial Neural Network models (ANN) for predicting the impact of the road traffic on the levels of PM10 concentration in London. Twin studies in conjunction with bivariate polar plots were used to identify and estimate the contribution of road traffic and other sources of PM10 at the monitoring sites. The road traffic was found to have contributed between 24% and 62% of the hourly average roadside PM10 concentrations. The ANN models performed well in predicting the road contributions with their R-values ranging between 0.6 and 0.9, FAC2 between 0.6 and 0.95, and the normalised mean bias between 0.01 and 0.11. The hourly emission rates of the vehicles were found to be the most contributing input variables to the outputs of the ANN models followed by background PM10, gaseous pollutants and meteorological variables respectively.

[1]  Pedro G. Lind,et al.  Air quality prediction using optimal neural networks with stochastic variables , 2013, 1307.3134.

[2]  Matthias Ketzel,et al.  Particle and trace gas emission factors under urban driving conditions in Copenhagen based on street and roof-level observations , 2003 .

[3]  Kim N. Dirks,et al.  Development of an ANN-based air pollution forecasting system with explicit knowledge through sensitivity analysis , 2014 .

[4]  Alison S. Tomlin,et al.  A field study of factors influencing the concentrations of a traffic-related pollutant in the vicinity of a complex urban junction , 2009 .

[5]  Shifei Ding,et al.  An optimizing BP neural network algorithm based on genetic algorithm , 2011, Artificial Intelligence Review.

[6]  Max Kuhn,et al.  The caret Package , 2007 .

[7]  Shikha Gupta,et al.  Identifying pollution sources and predicting urban air quality using ensemble learning methods , 2013 .

[8]  C. Willmott ON THE VALIDATION OF MODELS , 1981 .

[9]  M. Katz Validation of models , 2006 .

[10]  Alan M. Jones,et al.  Field study of the influence of meteorological factors and traffic volumes upon suspended particle mass at urban roadside sites of differing geometries , 2004 .

[11]  W. Nie,et al.  Airborne fine particulate pollution in Jinan, China: Concentrations, chemical compositions and influence on visibility impairment , 2012 .

[12]  B. Brunekreef,et al.  Effects of long-term exposure to traffic-related air pollution on respiratory and cardiovascular mortality in the Netherlands: the NLCS-AIR study. , 2009, Research report.

[13]  C. Willmott Some Comments on the Evaluation of Model Performance , 1982 .

[14]  Min Zhang,et al.  Heme oxygenase-1 protects endothelial cells from the toxicity of air pollutant chemicals. , 2015, Toxicology and applied pharmacology.

[15]  P K Hopke,et al.  Source apportionment of size resolved particulate matter at a European air pollution hot spot. , 2015, The Science of the total environment.

[16]  I. Barmpadimos,et al.  Influence of meteorology on PM 10 trends and variability in Switzerland from 1991 to 2008 , 2010 .

[17]  Hung-Lung Chiang,et al.  Pollutant constituents of exhaust emitted from light-duty diesel vehicles , 2012 .

[18]  S. Samarasinghe,et al.  Complex time series analysis of PM10 and PM2.5 for a coastal site using artificial neural network modelling and k-means clustering , 2014 .

[19]  Christopher M. Bishop,et al.  Neural networks for pattern recognition , 1995 .

[20]  R. Harrison,et al.  Estimation of the contribution of road traffic emissions to particulate matter concentrations from field measurements: A review , 2013 .

[21]  J. Thundiyil,et al.  Clearing the Air: A Review of the Effects of Particulate Matter Air Pollution on Human Health , 2011, Journal of Medical Toxicology.

[22]  Russell G. Death,et al.  An accurate comparison of methods for quantifying variable importance in artificial neural networks using simulated data , 2004 .

[23]  Fatih Taşpınar,et al.  Improving artificial neural network model predictions of daily average PM10 concentrations by applying principle component analysis and implementing seasonal models , 2015, Journal of the Air & Waste Management Association.

[24]  Yu Xue,et al.  Prediction of particulate matter at street level using artificial neural networks coupling with chaotic particle swarm optimization algorithm , 2014 .

[25]  Iratxe Uria-Tellaetxe,et al.  Conditional bivariate probability function for source identification , 2014, Environ. Model. Softw..

[26]  J. Morin,et al.  On-road measurements of particle number concentrations and size distributions in urban and tunnel environments , 2004 .

[27]  Aranildo R. Lima,et al.  Nonlinear regression in environmental sciences by support vector machines combined with evolutionary strategy , 2013, Comput. Geosci..

[28]  Hui Li,et al.  Evolutionary artificial neural networks: a review , 2011, Artificial Intelligence Review.

[29]  S. Vardoulakis,et al.  Levels, sources and seasonality of coarse particles (PM10–PM2.5) in three European capitals – Implications for particulate pollution control , 2012 .

[30]  David C. Carslaw,et al.  Characterising and understanding emission sources using bivariate polar plots and k-means clustering , 2013, Environ. Model. Softw..

[31]  Roy M. Harrison,et al.  Estimation of the emission factors of particle number and mass fractions from traffic at a site where mean vehicle speeds vary over short distances , 2006 .

[32]  Mohamed Abdel-Aty,et al.  A study on crashes related to visibility obstruction due to fog and smoke. , 2011, Accident; analysis and prevention.

[33]  D. Derwent,et al.  Evaluating the Performance of Air Quality Models , 2010 .

[34]  N. Pérez,et al.  Neural network model for the prediction of PM10 daily concentrations in two sites in the Western Mediterranean. , 2013, The Science of the total environment.

[35]  Julian D. Olden,et al.  Illuminating the “black box”: a randomization approach for understanding variable contributions in artificial neural networks , 2002 .

[36]  Roy M. Harrison,et al.  Quantification of air quality impacts of London Heathrow Airport (UK) from 2005 to 2012 , 2015 .

[37]  M. Ragosta,et al.  Input strategy analysis for an air quality data modelling procedure at a local scale based on neural network , 2015, Environmental Monitoring and Assessment.

[38]  M. Bell,et al.  Detecting and quantifying aircraft and other on-airport contributions to ambient nitrogen oxides in the vicinity of a large international airport , 2006 .