Plasmonic nanostructures for broadband solar absorption based on the intrinsic absorption of metals

Abstract In this study, several common plasmonic metals were compared for the development of a broadband absorber. It was found that a broadband absorption region, from 300 nm to 1500 nm, with average values of 89.9%, 91.0%, and 91.6%, was obtained for Ni, Ti, and W absorbers with high imaginary-part permittivities, respectively. The absorption peaks of Ag, Au, and Cu absorbers with low imaginary-part permittivities were mainly in a narrow visible region while the strong magnetic resonance was obtained in the broadband region. A detailed analysis indicated that the intrinsic absorption properties of the metal had a large effect on the broadband absorption ability of the simple-structure absorber and the metal with the high-imaginary-part-permittivity can reach a broadband absorption by the intrinsic absorption without enhanced magnetic resonance. Therefore, the high-imaginary-part-permittivity metal Ni was chosen to fabricate a broadband absorber; the geometric parameters of the Ni absorber were investigated by three-dimensional full-wave simulations to obtain a high-performance absorber. The detailed analysis indicated that the broadband-absorption mechanism can be attributed to the coupling effect of surface plasmon resonance, magnetic resonance, and intrinsic absorption of Ni. A high-performance solar absorber was proposed using Ni disks with two different sizes; the total solar thermal conversion efficiencies reached the values of 0.8909 and 0.8326 at operating temperatures of 800 K and 1000 K, respectively.

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