Auxiliary material Text S1 for "Absorbing aerosols over Asia: A Geophysical Fluid Dynamics Laboratory general circulation model sensitivity study of model response to aerosol optical depth and aerosol absorption"

[1] Forcing by absorbing atmospheric black carbon (BC) tends to heat the atmosphere, cool the surface, and reduce the surface latent and sensible heat fluxes. BC aerosol can have a large impact on regional climates and the hydrologic cycle. However, significant uncertainties remain concerning the increases in (1) the total amount of all aerosol species and (2) the amount of aerosol absorption that may have occurred over the 1950–1990 period. Focusing on south and east Asia, the sensitivity of a general circulation model's climate response (with prescribed sea surface temperatures and aerosol distributions) to such changes is investigated by considering a range of both aerosol absorption and aerosol extinction optical depth increases. We include direct and semidirect aerosol effects only. Precipitation changes are less sensitive to changes in aerosol absorption optical depth at lower aerosol loadings. At higher-extinction optical depths, low-level convergence and increases in vertical velocity overcome the stabilizing effects of absorbing aerosols and enhance the monsoonal circulation and precipitation in northwestern India. In contrast, the presence of increases in only scattering aerosols weakens the monsoonal circulation and inhibits precipitation here. Cloud amount changes can enhance or counteract surface solar flux reduction depending on the aerosol loading and absorption, with the changes also influencing the surface temperature and the surface energy balance. The results have implications for aerosol reduction strategies in the future that seek to mitigate air pollution concerns. At higher optical depths, if absorbing aerosol is present, reduction of scattering aerosol alone has a reduced effect on precipitation changes, implying that reductions in BC aerosols should be undertaken at the same time as reductions in sulfate aerosols.

[1]  Jean-Francois Lamarque,et al.  Multimodel projections of climate change from short‐lived emissions due to human activities , 2008 .

[2]  Kirsten L. Findell,et al.  Strong sensitivity of late 21st century climate to projected changes in short-lived air pollutants , 2008 .

[3]  V. Ramanathan,et al.  Global and regional climate changes due to black carbon , 2008 .

[4]  Hideaki Takenaka,et al.  Aerosol radiative characteristics at Gosan, Korea, during the Atmospheric Brown Cloud East Asian Regional Experiment 2005 , 2007 .

[5]  W. Hao,et al.  Aerosol single scattering albedo estimated across China from a combination of ground and satellite measurements , 2007 .

[6]  Vincent R. Gray Climate Change 2007: The Physical Science Basis Summary for Policymakers , 2007 .

[7]  L. Horowitz Past, present, and future concentrations of tropospheric ozone and aerosols: Methodology, ozone evaluation, and sensitivity to aerosol wet removal , 2006 .

[8]  V. Ramaswamy,et al.  Evaluation of aerosol distribution and optical depth in the Geophysical Fluid Dynamics Laboratory coupled model CM2.1 for present climate , 2006 .

[9]  Ka-Ming Lau,et al.  Observational relationships between aerosol and Asian monsoon rainfall, and circulation , 2006 .

[10]  Vincent R. Gray Temperature Trends in the Lower Atmosphere , 2006 .

[11]  Y. Gu Climatic effects of different aerosol types in China simulated , 2006 .

[12]  P. Jones,et al.  Uncertainty estimates in regional and global observed temperature changes: A new data set from 1850 , 2006 .

[13]  Chunsheng Zhao,et al.  A possible positive feedback of reduction of precipitation and increase in aerosols over eastern central China , 2006 .

[14]  V. Ramanathan,et al.  Weakening of North Indian SST Gradients and the Monsoon Rainfall in India and the Sahel , 2006 .

[15]  Differing regional responses to a perturbation in solar cloud absorption in the SKYHI general circulation model , 2006 .

[16]  R. Sagar,et al.  Aerosol characteristics at a high‐altitude location in central Himalayas: Optical properties and radiative forcing , 2006, physics/0603046.

[17]  T. Iwasaki,et al.  A GCM Study on the Roles of the Seasonal Marches of the SST and Land-Sea Thermal Contrast in the Onset of the Asian Summer Monsoon , 2006 .

[18]  K. Lau,et al.  Asian summer monsoon anomalies induced by aerosol direct forcing : the role of the Tibetan Plateau , 2006 .

[19]  R. Dickinson,et al.  Direct and indirect effects of anthropogenic aerosols on regional precipitation over east Asia , 2005 .

[20]  John H. Seinfeld,et al.  Climate response of direct radiative forcing of anthropogenic black carbon , 2005 .

[21]  T. Nakajima,et al.  Aerosol radiative forcing over east Asia determined from ground-based solar radiation measurements : Global aerosol system , 2005 .

[22]  Glen Lesins,et al.  Contribution of Changes in Sea Surface Temperature and Aerosol Loading to the Decreasing Precipitation Trend in Southern China , 2005 .

[23]  Q. Fu,et al.  Satellite‐derived vertical dependence of tropical tropospheric temperature trends , 2005 .

[24]  J. Kiehl,et al.  Atmospheric brown clouds: impacts on South Asian climate and hydrological cycle. , 2005, Proceedings of the National Academy of Sciences of the United States of America.

[25]  S. Tripathi,et al.  Aerosol black carbon radiative forcing at an industrial city in northern India , 2005 .

[26]  Q. Hu,et al.  Regulation of Tibetan Plateau heating on variation of Indian summer monsoon in the last two millennia , 2005 .

[27]  S. Klein,et al.  The new GFDL global atmosphere and land model AM2-LM2: Evaluation with prescribed SST simulations , 2004 .

[28]  B. Anderson Investigation of a Large-Scale Mode of Ocean-Atmosphere Variability and Its Relation to Tropical Pacific Sea Surface Temperature Anomalies , 2004 .

[29]  Shian‐Jiann Lin A “Vertically Lagrangian” Finite-Volume Dynamical Core for Global Models , 2004 .

[30]  Barry J. Huebert,et al.  Size distributions and mixtures of dust and black carbon aerosol in Asian outflow: Physiochemistry and optical properties , 2004 .

[31]  C. Fu,et al.  Simulation of the radiative effect of black carbon aerosols and the regional climate responses over China , 2004 .

[32]  Piers M. Forster,et al.  The semi‐direct aerosol effect: Impact of absorbing aerosols on marine stratocumulus , 2004 .

[33]  Igor A. Podgorny,et al.  The direct observations of large aerosol radiative forcing in the Himalayan region , 2004 .

[34]  J. Hansen,et al.  Soot climate forcing via snow and ice albedos. , 2004, Proceedings of the National Academy of Sciences of the United States of America.

[35]  F. Valero,et al.  Surface aerosol radiative forcing at Gosan during the ACE‐Asia campaign , 2003 .

[36]  T. Takemura,et al.  Significance of direct and indirect radiative forcings of aerosols in the East China Sea region , 2003 .

[37]  J. Seinfeld,et al.  A model for the radiative forcing during ACE-Asia derived from CIRPAS Twin Otter and R/V Ronald H. Brown data and comparison with observations , 2003 .

[38]  Young-Joon Kim,et al.  An overview of ACE‐Asia: Strategies for quantifying the relationships between Asian aerosols and their climatic impacts , 2003 .

[39]  Martin Wild,et al.  Inaugural Article by a Recently Elected Academy Member , 2003 .

[40]  P. Quinn,et al.  Influence of relative humidity on aerosol radiative forcing: An ACE‐Asia experiment perspective , 2003 .

[41]  V. Ramaswamy,et al.  Sensitivity of the atmospheric lapse rate to solar cloud absorption in a radiative‐convective model , 2003 .

[42]  J. Hansen,et al.  Climate Effects of Black Carbon Aerosols in China and India , 2002, Science.

[43]  V. Ramanathan,et al.  Effects of the south Asian absorbing haze on the northeast monsoon and surface-air heat exchange , 2002 .

[44]  S. Babu,et al.  Aerosol radiative forcing due to enhanced black carbon at an urban site in India , 2002 .

[45]  Thomas M. Smith,et al.  An Improved In Situ and Satellite SST Analysis for Climate , 2002 .

[46]  J. Houghton,et al.  Climate change 2001 : the scientific basis , 2001 .

[47]  E. Feil,et al.  Climate Effects of Black Carbon Aerosols in China and India , 2002 .

[48]  V. Ramanathan,et al.  Aerosols, Climate, and the Hydrological Cycle , 2001, Science.

[49]  Glenn E. Shaw,et al.  Indian Ocean Experiment: An integrated analysis of the climate forcing and effects of the great Indo-Asian haze , 2001 .

[50]  L. Weiliang,et al.  Characteristics of the spatial distribution and yearly variation of aerosol optical depth over China in last 30 years , 2001 .

[51]  T. Eck,et al.  An emerging ground-based aerosol climatology: Aerosol optical depth from AERONET , 2001 .

[52]  W. Collins,et al.  Simulating aerosols using a chemical transport model with assimilation of satellite aerosol retrievals: Methodology for INDOEX , 2001 .

[53]  Tim Li,et al.  Interannual and Interdecadal Variations of the East Asian Summer Monsoon and Tropical Pacific SSTs. Part I: Roles of the Subtropical Ridge , 2000 .

[54]  K. Shine Radiative Forcing of Climate Change , 2000 .

[55]  S. K. Satheesh,et al.  Large differences in tropical aerosol forcing at the top of the atmosphere and Earth's surface , 2000, Nature.

[56]  W. Malm,et al.  Effects of mixing on extinction by carbonaceous particles , 1999 .

[57]  Ramaswamy,et al.  Tropospheric Aerosol Climate Forcing in Clear-Sky Satellite Observations over the Oceans. , 1999, Science.

[58]  V. Ramaswamy,et al.  Global sensitivity studies of the direct radiative forcing due to anthropogenic sulfate and black carbon aerosols , 1998 .

[59]  J. Hansen,et al.  Radiative forcing and climate response , 1997 .

[60]  V. Ramaswamy,et al.  Sensitivity of simulated global climate to perturbations in low cloud microphysical properties. Part II: Spatially localized perturbations , 1996 .

[61]  M. Yanai,et al.  The onset and interannual variability of the Asian summer monsoon in relation to land-sea thermal contrast , 1996 .

[62]  Parameterization of the solar radiative characteristics of low clouds and studies with a general circulation model , 1995 .

[63]  G. Boer Climate change and the regulation of the surface moisture and energy budgets , 1993 .

[64]  S. Manabe,et al.  Cloud Feedback Processes in a General Circulation Model , 1988 .

[65]  J. Coakley,et al.  Response of the NCAR Community Climate Model to the Radiative Forcing by the Naturally Occurring Tropospheric Aerosol , 1985 .

[66]  J. Kiehl,et al.  Sensitivities of the radiative forcing due to large loadings of smoke and dust aerosols , 1985 .

[67]  Robert D. Cess,et al.  Nuclear war: Illustrative effects of atmospheric smoke and dust upon solar radiation , 1985 .

[68]  J. Peixoto,et al.  Physics of climate , 1984 .

[69]  J. W. Fitzgerald Approximation Formulas for the Equilibrium Size of an Aerosol Particle as a Function of Its Dry Size and Composition and the Ambient Relative Humidity , 1975 .

[70]  P. Chyacutelek,et al.  Aerosols and climate. , 1974 .

[71]  J. Coakley,et al.  Aerosols and Climate , 1974, Science.