Magnetic Field Effect on Thermal, Dielectric, and Viscous Properties of a Transformer Oil-Based Magnetic Nanofluid

Progress in electrical engineering puts a greater demand on the cooling and insulating properties of liquid media, such as transformer oils. To enhance their performance, researchers develop various nanofluids based on transformer oils. In this study, we focus on novel commercial transformer oil and a magnetic nanofluid containing iron oxide nanoparticles. Three key properties are experimentally investigated in this paper. Thermal conductivity was studied by a transient plane source method dependent on the magnetic volume fraction and external magnetic field. It is shown that the classical effective medium theory, such as the Maxwell model, fails to explain the obtained results. We highlight the importance of the magnetic field distribution and the location of the thermal conductivity sensor in the analysis of the anisotropic thermal conductivity. Dielectric permittivity of the magnetic nanofluid, dependent on electric field frequency and magnetic volume fraction, was measured by an LCR meter. The measurements were carried out in thin sample cells yielding unusual magneto-dielectric anisotropy, which was dependent on the magnetic volume fraction. Finally, the viscosity of the studied magnetic fluid was experimentally studied by means of a rheometer with a magneto-rheological device. The measurements proved the magneto-viscous effect, which intensifies with increasing magnetic volume fraction.

[1]  E. Shojaeizadeh,et al.  Magnetoviscous effect investigation of water based Mn-Zn Fe2O4 magnetic nanofluid under the influence of magnetic field: An experimental study , 2019, Journal of Magnetism and Magnetic Materials.

[2]  Y. Luengo,et al.  Rheological behavior of magnetic colloids in the borderline between ferrofluids and magnetorheological fluids , 2019, Journal of Rheology.

[3]  D. Jing,et al.  Time-dependent scattering of incident light of various wavelengths in ferrofluids under external magnetic field , 2018 .

[4]  C. Marin,et al.  Dependence on the temperature of the activation energy in the dielectric relaxation processes for ferrofluids in low-frequency field , 2002 .

[5]  A. Turgut,et al.  Effect of external magnetic field on thermal conductivity and viscosity of magnetic nanofluids: a review , 2019, Materials Research Express.

[6]  M. Rajňák,et al.  Electrode polarization and unusual magnetodielectric effect in a transformer oil-based magnetic nanofluid thin layer. , 2017, The Journal of chemical physics.

[7]  M. Rajňák,et al.  Transformer oil-based magnetic nanofluid with high dielectric losses tested for cooling of a model transformer , 2019, IEEE Transactions on Dielectrics and Electrical Insulation.

[8]  O. Marinică,et al.  The influence of particle clustering on the rheological properties of highly concentrated magnetic nanofluids. , 2012, Journal of colloid and interface science.

[9]  K. Parekh,et al.  Maneuvering thermal conductivity of magnetic nanofluids by tunable magnetic fields , 2015 .

[10]  M. Rajňák,et al.  Dielectric-spectroscopy approach to ferrofluid nanoparticle clustering induced by an external electric field. , 2014, Physical review. E, Statistical, nonlinear, and soft matter physics.

[11]  Alexandru M. Morega,et al.  Magnetic Nanofluid Applications in Electrical Engineering , 2013, IEEE Transactions on Magnetics.

[12]  Chao Tang,et al.  Review of Research Progress on the Electrical Properties and Modification of Mineral Insulating Oils Used in Power Transformers , 2018 .

[13]  I. Fofana 50 years in the development of insulating liquids , 2013, IEEE Electrical Insulation Magazine.

[14]  S. Odenbach,et al.  Rheological properties of magnetic fluids and their microstructural background , 2007 .

[15]  P. Meakin,et al.  Effect of aggregation on thermal conduction in colloidal nanofluids , 2006 .

[16]  Jong-Chul Lee,et al.  The increased dielectric breakdown voltage of transformer oil-based nanofluids by an external magnetic field , 2012 .

[17]  C. Altan,et al.  Enhancement of thermal conductivity upon application of magnetic field to Fe3O4 nanofluids , 2011 .

[18]  N. Nguyen,et al.  Onset of thermomagnetic convection around a vertically oriented hot-wire in ferrofluid , 2018, Journal of Magnetism and Magnetic Materials.

[19]  Markus Zahn,et al.  Effects of nanoparticle charging on streamer development in transformer oil-based nanofluids , 2010 .

[20]  A. Gavili,et al.  The thermal conductivity of water base ferrofluids under magnetic field , 2012 .

[21]  Qiang Li,et al.  Experimental investigations on transport properties of magnetic fluids , 2005 .

[22]  A. Spanoudaki,et al.  Frequency dependence of dielectric anisotropy in ferrofluids , 2002 .

[23]  B. Raj,et al.  Enhancement of thermal conductivity in magnetite based nanofluid due to chainlike structures , 2007 .

[24]  M. Rajňák,et al.  Effect of magnetic nanoparticles on partial discharges in transformer oil , 2020 .

[25]  M. Rajňák,et al.  Toward Apparent Negative Permittivity Measurement in a Magnetic Nanofluid with Electrically Induced Clusters , 2019, Physical Review Applied.

[26]  K. Chattopadhyay,et al.  Amorphous graphene – Transformer oil nanofluids with superior thermal and insulating properties , 2018, Carbon.

[27]  Doina Bica,et al.  Magnetic nanoparticles and concentrated magnetic nanofluids: Synthesis, properties and some applications , 2007 .

[28]  Youn-J. Kim,et al.  Thermomagnetic Convection of Ferrofluid in an Enclosure Channel with an Internal Magnetic Field , 2019, Micromachines.

[29]  F. R. Cunha,et al.  The influence of dipolar particle interactions on the magnetization and the rotational viscosity of ferrofluids , 2019, Physics of Fluids.

[30]  Yanmin Wang,et al.  Heat transfer enhancement by magnetic nanofluids—A review , 2013 .

[31]  B. Sundén,et al.  Convective heat transfer performance of aggregate-laden nanofluids , 2016 .

[32]  Sarit K. Das,et al.  Thermal conductivity enhancement of nanofluids containing graphene nanosheets , 2011 .

[33]  Jacob Fish,et al.  Effect of aggregation and interfacial thermal resistance on thermal conductivity of nanocomposites and colloidal nanofluids , 2008 .

[34]  K. Parekh,et al.  Magnetic field induced enhancement in thermal conductivity of magnetite nanofluid , 2010 .

[35]  W. Sima,et al.  A Promising Nano-Insulating-Oil for Industrial Application: Electrical Properties and Modification Mechanism , 2019, Nanomaterials.

[36]  Baldev Raj,et al.  Magnetically controllable nanofluid with tunable thermal conductivity and viscosity , 2009 .

[37]  Stefan Odenbach,et al.  Magnetoviscous effects in ferrofluids , 2002 .

[38]  M. Rajňák,et al.  Experimental study of AC breakdown strength in ferrofluid during thermal aging , 2018, Journal of Magnetism and Magnetic Materials.