Lateral forces during manipulation of a single C60 molecule on the Si()-2×1 surface

Abstract A method to measure lateral manipulation forces of a single molecule or a cluster was developed by combining scanning tunneling microscopy with a special lateral force sensor. The tunneling current and lateral force associated with manipulation of a single C 60 molecule on the Si(0 0 1)-2×1 surface were measured simultaneously during raster scanning of the probe. From the measured lateral force profiles the molecular hopping motion was analyzed and an estimate of the elastic energy stored in the molecule was determined.

[1]  D. Sarid,et al.  Intramolecular features of individual C60 molecules on Si(100) observed by STM , 1996 .

[2]  Shizuka Nakano,et al.  Atomic Force Microscopy Cantilevers for Sensitive Lateral Force Detection , 1999 .

[3]  D. Kondo,et al.  Bonding nature of C60 adsorbed on Si(111) 7 × 7 and Si(100) 2 × 1 surfaces studied by HREELS and PES , 1999 .

[4]  D. Sarid,et al.  An STM study of C60 adsorption on Si(100)-(2 × 1) surfaces: from physisorption to chemisorption , 1995 .

[5]  J. M. Martín,et al.  Superlubricity of molybdenum disulphide. , 1993, Physical review. B, Condensed matter.

[6]  A. Dunn,et al.  C60-TERMINATED SI SURFACES : CHARGE TRANSFER, BONDING, AND CHEMICAL PASSIVATION , 1998 .

[7]  M. Pachter,et al.  Anisotropic stress and molecular moduli of C60 , 1992 .

[8]  Sakurai,et al.  Adsorption of C60 and C84 on the Si(100)2 x 1 surface studied by using the scanning tunneling microscope. , 1993, Physical review. B, Condensed matter.

[9]  F. Besenbacher,et al.  Kinetics of island diffusion on Cu(111) and Ag(111) studied with variable-temperature STM , 2000 .

[10]  M. Ho,et al.  Direct observation of electromigration of Si magic clusters on Si(111) surfaces. , 2000, Physical review letters.

[11]  D. Sanvitto,et al.  DIRECT EVIDENCE OF C60 CHEMICAL BONDING ON SI(100) , 1999 .

[12]  D. Eigler,et al.  Positioning single atoms with a scanning tunnelling microscope , 1990, Nature.

[13]  Gerd Meyer,et al.  BASIC STEPS OF LATERAL MANIPULATION OF SINGLE ATOMS AND DIATOMIC CLUSTERS WITH A SCANNING TUNNELING MICROSCOPE TIP , 1997 .

[14]  Hirano,et al.  Anisotropy of frictional forces in muscovite mica. , 1991, Physical review letters.

[15]  N. Bartelt,et al.  Alloying at surfaces by the migration of reactive two-dimensional islands. , 2000, Science.

[16]  Philip Moriarty,et al.  Translation, rotation and removal of C60 on Si(100)-2 × 1 using anisotropic molecular manipulation , 1998 .

[17]  H. Reiss Rotation and Translation of Islands in the Growth of Heteroepitaxial Films , 1968 .

[18]  R. Kaneko,et al.  Observation of Superlubricity by Scanning Tunneling Microscopy , 1997 .

[19]  G. Binnig,et al.  Scanning tunneling microscopy , 1984 .