High-resolution 3D fabric and porosity model in a tight gas sandstone reservoir:A new approach to investigate microstructures from mm- to nm-scale combining argon beam cross-sectioning and SEM imaging

Abstract The development of new technologies to enhance tight gas reservoir productivity could strongly benefit from a better resolution and imaging of the porosity. Numerous methods are available to characterize sandstone porosity. However, imaging of pore space at scales below 1 μm in tight gas sands remains difficult due to limits in resolution and sample preparation. We explored the use of high resolution SEM in combination with argon ion beam cross sectioning (BIB, Broad Ion Beam) to prepare smooth, and damage-free, true-2D surfaces of tight gas sandstone core samples from the Permian Rotliegend in Germany, to image porosity down to 10 nm. The quality of cross-sections allows measuring porosity at pore scale, and describing the bulk porosity by defining different regions with characteristic pore morphology and pore size distribution. Serial cross sectioning of samples produces a 3D model of the porous network. We present a model of fabric and porosity at 2 different scales: the scale of sand grains and the scale of the clay grains in the intergranular volume.

[1]  N. F. Djabbarah,et al.  Whole Core Analysis - Experience and Challenges , 2005 .

[2]  Beatriz Menéndez,et al.  Confocal scanning laser microscopy applied to the study of pore and crack networks in rocks , 2001 .

[3]  R. Wepf,et al.  3D-microstructure analysis of hydrated bentonite with cryo-stabilized pore water , 2010 .

[4]  A. Bashari DIAGENESIS AND RESERVOIR DEVELOPMENT OF SANDSTONES IN THE TRIASSIC REWAN GROUP, BOWEN BASIN, AUSTRALIA , 1998 .

[5]  U. Schwertmann,et al.  Influence of Hematite on the Color of Red Beds , 1987 .

[6]  Qian Fang,et al.  Computer simulations of fluid flow in sediment: From images to permeability , 2010 .

[7]  P. Nadeau Fundamental particles and the advancement of geosciences; response to Implications of TEM data for the concept of fundamental particles , 1998 .

[8]  R. Schöner Comparison of Rotliegend sandstone diagenesis from the northern and southern margin of the North German Basin, and implications for the importance of organic maturation and migration , 2006 .

[9]  E. Favvas,et al.  Characterization of carbonate rocks by combination of scattering, porosimetry and permeability techniques , 2009 .

[10]  B. Velde,et al.  Changes in Particle Morphology During Illitization: An Experimental Study , 1993 .

[11]  T. Mccann The Rotliegend of the NE German Basin; background and prospectivity , 1998, Petroleum Geoscience.

[12]  L. Macchi A review of sandstone illite cements and aspects of their significance to hydrocarbon exploration and development , 1987 .

[13]  N. Erdman,et al.  Precise SEM Cross Section Polishing via Argon Beam Milling , 2006, Microscopy Today.

[14]  B. Law,et al.  Introduction to unconventional petroleum systems , 2002 .

[15]  Susanne Nelskamp,et al.  Dynamics of Complex Intracontinental Basins : The Central European Basin System , 2008 .

[16]  Peter Abram Relations between seismic signals and reservoir properties of deep gas reservoirs in Northwest-Germany -Wustrow member, Rotliegend , 2008 .

[17]  Djebbar Tiab,et al.  Petrophysics: Theory and Practice of Measuring Reservoir Rock and Fluid Transport Properties , 1996 .

[18]  A. Hildenbrand,et al.  Investigation of the morphology of pore space in mudstones—first results , 2003 .

[19]  Yelena Sholokhova,et al.  Network Flow Modeling via Lattice-Boltzmann Based Channel Conductance. Prediction of Relative Permeability in Primary Drainage. , 2009 .

[20]  Colin R. Ward,et al.  Use of mineralogical analysis in geotechnical assessment of rock strata for coal mining , 2005 .

[21]  Lorenz Holzer,et al.  Review of FIB tomography , 2012 .

[22]  J. Kantorowicz The influence of variations in illite morphology on the permeability of Middle Jurassic Brent Group sandstones, Cormorant Field, UK North Sea , 1990 .

[23]  János Urai,et al.  Morphology of the pore space in claystones - evidence from BIB/FIB ion beam sectioning and cryo-SEM observations , 2009 .

[24]  K. Ziegler Clay minerals of the Permian Rotliegend Group in the North Sea and adjacent areas , 2006, Clay Minerals.

[25]  T. Mccann SANDSTONE COMPOSITION AND PROVENANCE OF THE ROTLIEGEND OF THE NE GERMAN BASIN , 1998 .

[26]  R. Wepf,et al.  Cryo‐FIB‐nanotomography for quantitative analysis of particle structures in cement suspensions , 2007, Journal of microscopy.

[27]  Christoph Börmann,et al.  Structural and sedimentological analysis of an early Late Rotliegendes graben based on 3D seismic and well log data, German North Sea , 2006, Petroleum Geoscience.

[28]  J. L. Uraib,et al.  Investigation of the morphology of pore space in mudstones — first results , 2003 .

[29]  Michael D. Abràmoff,et al.  Image processing with ImageJ , 2004 .

[30]  B. Humbel,et al.  Cryogenic vitrification and 3D serial sectioning using high resolution cryo‐FIB SEM technology for brine‐filled grain boundaries in halite: first results , 2008 .

[31]  R. Loucks,et al.  Morphology, Genesis, and Distribution of Nanometer-Scale Pores in Siliceous Mudstones of the Mississippian Barnett Shale , 2009 .

[32]  S. Rahman,et al.  Response of low-permeability, illitic sandstone to drilling and completion fluids , 1995 .

[33]  M. Eigner,et al.  The role of diagenetic studies in production operations , 1986, Clay Minerals.

[34]  T. E. Unander,et al.  Core damage effects on compaction behaviour , 1994 .

[35]  B. Haimson Micromechanisms of borehole instability leading to breakouts in rocks , 2007 .

[36]  R. Haszeldine,et al.  Fibrous illite in oilfield sandstones – a nucleation kinetic theory of growth , 2002 .

[37]  S. Baraka-Lokmanea,et al.  Application of complementary methods for more robust characterization of sandstone cores , 2008 .

[38]  K. Schulmann,et al.  Contrasting textural record of two distinct metamorphic events of similar P–T conditions and different durations , 2005 .

[39]  A. Meunier,et al.  Authigenic kaolin and illitic minerals during burial diagenesis of sandstones: a review , 2002, Clay Minerals.

[40]  J. Howell,et al.  Predicting distribution of remobilized aeolian facies using sub-surface data: the Weissliegend of the UK Southern North Sea , 2002, Petroleum Geoscience.

[41]  R. M. Pollastro Mineralogical and Morphological Evidence for the Formation of Illite at the Expense of Illite/Smectite , 1985 .

[42]  F. Chester,et al.  Mechanisms of compaction of quartz sand at diagenetic conditions , 2004 .

[43]  B. Velde,et al.  Illite: Origins, Evolution and Metamorphism , 2010 .

[44]  A. Bally Introduction to the petroleum geology of the North Sea , 1985 .

[45]  Dirk Gajewski,et al.  Dynamics of Complex Intracontinental Basins , 2008 .

[46]  R. Gaupp,et al.  On the origin of the Southern Permian Basin, Central Europe , 2000 .

[47]  R. Gaupp,et al.  Contrasting red bed diagenesis: the southern and northern margin of the Central European Basin , 2005 .

[48]  K. Glennie Development of N.W. Europe’s Southern Permian Gas Basin , 1986, Geological Society, London, Special Publications.

[49]  S. Holditch Tight Gas Sands , 2006 .

[50]  A. Hurst,et al.  Application of Back-Scattered Electron Microscopy to the Quantification of Clay Mineral Microporosity in Sandstones , 1991 .

[51]  Jeff Wilson,et al.  The Relationship Between Permeability and the Morphology of Diagenetic Illite in Reservoir Rocks , 1984 .

[52]  J. Dvorkin Digital rock physics bridges scales of measurement , 2009 .

[53]  K. Glennie Introduction to the petroleum geology of the North Sea , 1986 .

[54]  J. M. Tait,et al.  The conversion of smectite to illite during diagenesis: evidence from some illitic clays from bentonites and sandstones , 1985, Mineralogical Magazine.

[55]  U. Seemann DIAGENETICALLY FORMED INTERSTITIAL CLAY MINERALS AS A FACTOR IN ROTLIEGEND SANDSTONE RESERVOIR QUALITY IN THE DUTCH SECTOR OF THE NORTH SEA , 1979 .

[56]  M. Holz,et al.  Pore geometry of sandstone derived from pulsed field gradient NMR , 2006 .

[57]  J. Walzebuck,et al.  Diagenesis and Fluid Evolution of Deeply Buried Permian (Rotliegende) Gas Reservoirs, Northwest Germany , 1993 .

[58]  D. Tiab,et al.  Fluid-Rock Interactions , 2004 .

[59]  L. V. Vliet,et al.  Grain size stabilisation by dispersed graphite in a high-grade quartz mylonite: an example from Naxos (Greece) , 2003 .

[60]  T. Bushell Reservoir Geology of the Morecambe Field , 1986, Geological Society, London, Special Publications.