Evaluation of climate model aerosol seasonal and spatial variability over Africa using AERONET

Abstract. The sensitivity of climate models to the characterization of African aerosol particles is poorly understood. Africa is a major source of dust and biomass burning aerosols and this represents an important research gap in understanding the impact of aerosols on radiative forcing of the climate system. Here we evaluate the current representation of aerosol particles in the Conformal Cubic Atmospheric Model (CCAM) with ground-based remote retrievals across Africa, and additionally provide an analysis of observed aerosol optical depth at 550 nm (AOD550 nm) and Angstrom exponent data from 34 Aerosol Robotic Network (AERONET) sites. Analysis of the 34 long-term AERONET sites confirms the importance of dust and biomass burning emissions to the seasonal cycle and magnitude of AOD550 nm across the continent and the transport of these emissions to regions outside of the continent. In general, CCAM captures the seasonality of the AERONET data across the continent. The magnitude of modeled and observed multiyear monthly average AOD550 nm overlap within ±1 standard deviation of each other for at least 7 months at all sites except the Reunion St Denis Island site (Reunion St. Denis). The timing of modeled peak AOD550 nm in southern Africa occurs 1 month prior to the observed peak, which does not align with the timing of maximum fire counts in the region. For the western and northern African sites, it is evident that CCAM currently overestimates dust in some regions while others (e.g., the Arabian Peninsula) are better characterized. This may be due to overestimated dust lifetime, or that the characterization of the soil for these areas needs to be updated with local information. The CCAM simulated AOD550 nm for the global domain is within the spread of previously published results from CMIP5 and AeroCom experiments for black carbon, organic carbon, and sulfate aerosols. The model's performance provides confidence for using the model to estimate large-scale regional impacts of African aerosols on radiative forcing, but local feedbacks between dust aerosols and climate over northern Africa and the Mediterranean may be overestimated.

[1]  S. Piketh,et al.  Smoke and Clouds above the Southeast Atlantic: Upcoming Field Campaigns Probe Absorbing Aerosol’s Impact on Climate , 2016 .

[2]  Philippe Ciais,et al.  The status and challenge of global fire modelling , 2016 .

[3]  S. Archibald Managing the human component of fire regimes: lessons from Africa , 2016, Philosophical Transactions of the Royal Society B: Biological Sciences.

[4]  F. Guichard,et al.  The past, present and future of African dust , 2016, Nature.

[5]  Philip Stier,et al.  The importance of temporal collocation for the evaluation of aerosol models with observations , 2015 .

[6]  F. Guichard,et al.  Can we use surface wind fields from meteorological reanalyses for Sahelian dust emission simulations? , 2015 .

[7]  M. Chin,et al.  The fertilizing role of African dust in the Amazon rainforest: A first multiyear assessment based on data from Cloud‐Aerosol Lidar and Infrared Pathfinder Satellite Observations , 2015 .

[8]  Laurent Menut,et al.  Derivation of an observation-based map of North African dust emission , 2015 .

[9]  V. Cachorro,et al.  Aerosol characterization at the Saharan AERONET site Tamanrasset , 2014 .

[10]  A. Evan,et al.  Identification of a new dust‐stratocumulus indirect effect over the tropical North Atlantic , 2014 .

[11]  Gabriele Curci,et al.  The AeroCom evaluation and intercomparison of organic aerosol in global models , 2014, Atmospheric Chemistry and Physics.

[12]  D. N. Walters,et al.  Impacts of increasing the aerosol complexity in the Met Office global numerical weather prediction model , 2014 .

[13]  W. Landuyt,et al.  The vertical distribution of black carbon in CMIP5 models: Comparison to observations and the importance of convective transport , 2014 .

[14]  Shian-Jiann Lin,et al.  Atmospheric Sulfur Cycle Simulated in the Global Model Gocart: Model Description and Global Properties , 2013 .

[15]  B. DeAngelo,et al.  Bounding the role of black carbon in the climate system: A scientific assessment , 2013 .

[16]  J. Randerson,et al.  Global burned area and biomass burning emissions from small fires , 2012 .

[17]  Kerstin Schepanski,et al.  Comparing two years of Saharan dust source activation obtained by regional modelling and satellite observations , 2012 .

[18]  M. Chin,et al.  Host model uncertainties in aerosol radiative forcing estimates: results from the AeroCom Prescribed intercomparison study , 2012 .

[19]  S. Jeffrey,et al.  Aerosol- and greenhouse gas-induced changes in summer rainfall and circulation in the Australasian region: a study using single-forcing climate simulations , 2012 .

[20]  S. Jeffrey,et al.  Aerosol-induced changes in summer rainfall and circulation in the Australasian region: a study using single-forcing climate simulations , 2012 .

[21]  Dongxiao Zhang,et al.  Influence of African dust on ocean-atmosphere variability in the tropical Atlantic , 2011 .

[22]  Venkataraman Sivakumar,et al.  Aerosol climatology over South Africa based on 10 years of Multiangle Imaging Spectroradiometer (MISR) data , 2011 .

[23]  A. Thomson,et al.  The representative concentration pathways: an overview , 2011 .

[24]  Michael Schulz,et al.  Global dust model intercomparison in AeroCom phase I , 2011 .

[25]  A. Robinson,et al.  The influence of semi-volatile and reactive primary emissions on the abundance and properties of global organic aerosol , 2011 .

[26]  M. Pickering,et al.  Echinobothrium joshuai n. sp. (Cestoda: Diphyllidea) from the Roughnose Legskate, Cruriraja hulleyi (Rajiformes: Rajidae), off South Africa , 2011 .

[27]  N. Pérez,et al.  Transport of desert dust mixed with North African industrial pollutants in the subtropical Saharan Air Layer , 2011 .

[28]  R. Mitchell,et al.  Simulated enhancement of ENSO-related rainfall variability due to Australian dust , 2011 .

[29]  S. Piketh,et al.  Climatology of aerosol optical properties in Southern Africa , 2011 .

[30]  J. Thepaut,et al.  The ERA‐Interim reanalysis: configuration and performance of the data assimilation system , 2011 .

[31]  J. Randerson,et al.  Global fire emissions and the contribution of deforestation, savanna, forest, agricultural, and peat fires (1997-2009) , 2010 .

[32]  D. Roy,et al.  Southern African Fire Regimes as Revealed by Remote Sensing , 2010 .

[33]  C. Liousse,et al.  Simulation of the direct and semidirect aerosol effects on the southern Africa regional climate during the biomass burning season , 2010 .

[34]  P. V. Velthoven,et al.  Updated African biomass burning emission inventories in the framework of the AMMA-IDAF program, with an evaluation of combustion aerosols , 2010 .

[35]  R. Pinker,et al.  Radiative effects of aerosols in sub‐Sahel Africa: Dust and biomass burning , 2010 .

[36]  Adrian Chappell,et al.  Fertilizing the Amazon and equatorial Atlantic with West African dust , 2010 .

[37]  John F. B. Mitchell,et al.  The next generation of scenarios for climate change research and assessment , 2010, Nature.

[38]  Didier Tanré,et al.  Aerosol vertical distribution and optical properties over M'Bour (16.96 W; 14.39 N), Senegal from 2006 to 2008 , 2009 .

[39]  G. Kallos,et al.  African dust contributions to mean ambient PM10 mass-levels across the Mediterranean Basin , 2009 .

[40]  M. Tesfaye,et al.  Aerosol measurements over Southern Africa using LIDAR, satellite and sun-photometer , 2009 .

[41]  V. Ramaswamy,et al.  Evaluation of tropical and extratropical Southern Hemisphere African aerosol properties simulated by a climate model , 2009 .

[42]  Marcus Thatcher,et al.  Using a Scale-Selective Filter for Dynamical Downscaling with the Conformal Cubic Atmospheric Model , 2009 .

[43]  Yan Feng,et al.  Improved simulation of Australian climate and ENSO‐related rainfall variability in a global climate model with an interactive aerosol treatment , 2009 .

[44]  Victoria E. Cachorro,et al.  Airmass Classification and Analysis of Aerosol Types at El Arenosillo (Spain) , 2009 .

[45]  Gerard Capes,et al.  Overview of the Dust and Biomass‐burning Experiment and African Monsoon Multidisciplinary Analysis Special Observing Period‐0 , 2008 .

[46]  Paola Formenti,et al.  AMMA dust experiment: An overview of measurements performed during the dry season special observation period (SOP0) at the Banizoumbou (Niger) supersite , 2008 .

[47]  G. Roberts,et al.  Annual and diurnal african biomass burning temporal dynamics , 2008 .

[48]  Andreas Macke,et al.  Saharan dust transport and deposition towards the tropical northern Atlantic , 2008 .

[49]  P. Formenti,et al.  Evidence for large-scale transport of biomass burning aerosols from sunphotometry at a remote South African site , 2008 .

[50]  C. Simmer,et al.  Spectral aerosol optical properties from AERONET Sun-photometric measurements over West Africa , 2008 .

[51]  T. Eck,et al.  Spatial and temporal variability of column-integrated aerosol optical properties in the southern Arabian Gulf and United Arab Emirates in summer , 2008 .

[52]  Victoria E. Cachorro,et al.  Inventory of African desert dust events over the southwestern Iberian Peninsula in 2000-2005 with an AERONET Cimel Sun photometer , 2007 .

[53]  N. Nakicenovic,et al.  Scenarios of long-term socio-economic and environmental development under climate stabilization , 2007 .

[54]  Yan Feng,et al.  Have Australian rainfall and cloudiness increased due to the remote effects of Asian anthropogenic aerosols , 2007 .

[55]  Victoria E. Cachorro,et al.  Aerosol optical depth and Ångström exponent climatology at El Arenosillo AERONET site (Huelva, Spain) , 2007 .

[56]  M. Deeter,et al.  Satellite-observed pollution from Southern Hemisphere biomass burning. , 2006 .

[57]  C. Justice,et al.  Global distribution and seasonality of active fires as observed with the Terra and Aqua Moderate Resolution Imaging Spectroradiometer (MODIS) sensors , 2006 .

[58]  J. Penner,et al.  Global modeling of aerosol dynamics: Model description, evaluation, and interactions between sulfate and nonsulfate aerosols , 2005 .

[59]  J. Haywood,et al.  The direct radiative effect of biomass burning aerosols over southern Africa , 2005 .

[60]  C. Zender,et al.  Quantifying mineral dust mass budgets:Terminology, constraints, and current estimates , 2004 .

[61]  D. Streets,et al.  A technology‐based global inventory of black and organic carbon emissions from combustion , 2004 .

[62]  Mian Chin,et al.  Long-term simulation of global dust distribution with the GOCART model: correlation with North Atlantic Oscillation , 2004, Environ. Model. Softw..

[63]  J. Randerson,et al.  Continental-Scale Partitioning of Fire Emissions During the 1997 to 2001 El Niño/La Niña Period , 2003, Science.

[64]  J. Privette,et al.  Africa burning: A thematic analysis of the Southern African Regional Science Initiative (SAFARI 2000) , 2003 .

[65]  T. Berntsen,et al.  Modeling the solar radiative impact of aerosols from biomass burning during the Southern African Regional Science Initiative (SAFARI-2000) experiment , 2003 .

[66]  C. Justice,et al.  Seasonal to interannual variability of vegetation and fires at SAFARI 2000 sites inferred from advanced very high resolution radiometer time series data , 2003 .

[67]  Thomas F. Eck,et al.  Variability of biomass burning aerosol optical characteristics in southern Africa during the SAFARI , 2003 .

[68]  U. Lohmann,et al.  Simulation of the tropospheric sulfur cycle in a global model with a physically based cloud scheme , 2002 .

[69]  O. Torres,et al.  ENVIRONMENTAL CHARACTERIZATION OF GLOBAL SOURCES OF ATMOSPHERIC SOIL DUST IDENTIFIED WITH THE NIMBUS 7 TOTAL OZONE MAPPING SPECTROMETER (TOMS) ABSORBING AEROSOL PRODUCT , 2002 .

[70]  M. Chin,et al.  Sources and distributions of dust aerosols simulated with the GOCART model , 2001 .

[71]  T. Eck,et al.  An emerging ground-based aerosol climatology: Aerosol optical depth from AERONET , 2001 .

[72]  Alexander Smirnov,et al.  Cloud-Screening and Quality Control Algorithms for the AERONET Database , 2000 .

[73]  R. Van Dingenen,et al.  Chemical mass closure and assessment of the origin of the submicron aerosol in the marine boundary layer and the free troposphere at Tenerife during ACE-2 , 2000 .

[74]  M. Chin,et al.  Tropospheric sulfur simulation and sulfate direct radiative forcing in the Goddard Institute for Space Studies general circulation model , 1999 .

[75]  C. Liousse,et al.  Construction of a 1° × 1° fossil fuel emission data set for carbonaceous aerosol and implementation and radiative impact in the ECHAM4 model , 1999 .

[76]  Alexandros Papayannis,et al.  Characterization of the vertical structure of Saharan dust export to the Mediterranean basin , 1999 .

[77]  Ulrike Lohmann,et al.  Erratum: ``Prediction of the number of cloud droplets in the ECHAM GCM'' , 1999 .

[78]  C. Liousse,et al.  Contribution of the different aerosol species to the aerosol mass load and optical depth over the northeastern tropical Atlantic , 1999 .

[79]  A. Smirnov,et al.  AERONET-a federated instrument network and data archive for aerosol Characterization , 1998 .

[80]  François Dulac,et al.  Control of atmospheric export of dust from North Africa by the North Atlantic Oscillation , 1997, Nature.

[81]  M. Garstang,et al.  Large-Scale Recirculation of Air over Southern Africa , 1996 .

[82]  M. Garstang,et al.  Horizontal and vertical transport of air over southern Africa , 1996 .

[83]  B. Koffi,et al.  Seasonality of vegetation fires in Africa from remote sensing data and application to a global chemistry model , 1996 .

[84]  M. Garstang,et al.  AN AIR TRANSPORT CLIMATOLOGY FOR SUBTROPICAL SOUTHERN AFRICA , 1996 .

[85]  Didier Tanré,et al.  Satellite Climatology of Saharan Dust Outbreaks: Method and Preliminary Results , 1992 .

[86]  P. Crutzen,et al.  Biomass Burning in the Tropics: Impact on Atmospheric Chemistry and Biogeochemical Cycles , 1990, Science.

[87]  Corinne Le Quéré,et al.  Climate Change 2013: The Physical Science Basis , 2013 .

[88]  © Author(s) 2010. CC Attribution 3.0 License. Atmospheric Chemistry and Physics , 2010 .

[89]  J. Baldasano,et al.  Atmospheric Chemistry and Physics Aerosol Characterization in Northern Africa, Northeastern Atlantic, Mediterranean Basin and Middle East from Direct-sun Aeronet Observations , 2009 .

[90]  D. Holdstock Past, present--and future? , 2005, Medicine, conflict, and survival.

[91]  © Author(s) 2006. This work is licensed under a Creative Commons License. Atmospheric Chemistry and Physics , 2005 .

[92]  R. Martin,et al.  Interannual and seasonal variability of biomass burning emissions constrained by satellite observations , 2003 .

[93]  R. Jaenicke,et al.  Saharan dust transport over the North Atlantic Ocean , 1981 .

[94]  D. Meloni,et al.  © Author(s) 2006. This work is licensed under a Creative Commons License. Atmospheric Chemistry and Physics Aerosol optical properties at Lampedusa (Central Mediterranean). 1. Influence of transport and identification of different aerosol types , 2022 .