Reversible Fermi Level Tuning of a Sb₂Te₃ Topological Insulator by Structural Deformation.

For three-dimensional (3D) topological insulators that have a layered structure, strain was used to control critical physical properties. Here, we show that tensile strain decreases bulk carrier density while accentuating transport of topological surface state using temperature-dependent resistance and magneto-resistance measurements, terahertz-time domain spectroscopy and density functional theory calculations. The induced strain was confirmed by transmittance X-ray scattering measurements. The results show the possibility of reversible topological surface state device control using structural deformation.

[1]  Hai-Zhou Lu,et al.  Weak localization of bulk channels in topological insulator thin films , 2011, 1107.3959.

[2]  D. Hsieh Textures in Topological Insulators Observation of Unconventional Quantum Spin , 2009 .

[3]  Hong-Ying Zhai,et al.  Far-infrared optical conductivity gap in superconducting MgB2 films. , 2002, Physical review letters.

[4]  Q. Xue,et al.  Evidence for electron-electron interaction in topological insulator thin films , 2010, 1012.0271.

[5]  Pingxiong Yang,et al.  Growth and characterization of Sb2Te3 thin film deposited by pulsed laser method , 2013, Other Conferences.

[6]  H. D. Yang,et al.  THz Generation and Detection on Dirac Fermions in Topological Insulators , 2013, 1302.1087.

[7]  Jonghun Kim,et al.  Strain effects on in-plane conductance of the topological insulator Bi2Te3 , 2014 .

[8]  Xiao-Liang Qi,et al.  Aharonov-Bohm interference in topological insulator nanoribbons. , 2009, Nature materials.

[9]  C. Beenakker,et al.  Electrically detected interferometry of Majorana fermions in a topological insulator. , 2009, Physical review letters.

[10]  Yang Yang,et al.  Structure properties of BiFeO3 films studied by micro-Raman scattering , 2008 .

[11]  S. Sasaki,et al.  Achieving Surface Quantum Oscillations in Topological Insulator Thin Films of Bi2Se3 , 2012, Advanced materials.

[12]  Seung Jin Chae,et al.  Gate-controlled nonlinear conductivity of Dirac fermion in graphene field-effect transistors measured by terahertz time-domain spectroscopy. , 2012, Nano letters.

[13]  A. I. Larkin,et al.  Spin-Orbit Interaction and Magnetoresistance in the Two Dimensional Random System , 1980 .

[14]  Tae Hyeon Kim,et al.  Phase Transformation through Metastable Structures in Atomically Controlled Se/Sb MultiLayers , 2011 .

[15]  David J. Singh,et al.  Seebeck and figure of merit enhancement in nanostructured antimony telluride by antisite defect suppression through sulfur doping. , 2012, Nano letters.

[16]  Xi Dai,et al.  Topological insulators in Bi2Se3, Bi2Te3 and Sb2Te3 with a single Dirac cone on the surface , 2009 .

[17]  Tohru Suemoto,et al.  Photoinduced metallic state in VO2 proved by the terahertz pump-probe spectroscopy , 2008 .

[18]  Zhongfan Liu,et al.  Selective‐Area Van der Waals Epitaxy of Topological Insulator Grid Nanostructures for Broadband Transparent Flexible Electrodes , 2013, Advanced materials.

[19]  Influence of strain on anisotropic thermoelectric transport in Bi2Te3and Sb2Te3 , 2011, 1108.1304.

[20]  J. Jia Topological insulators: Strain away , 2014 .

[21]  T. Yokoyama,et al.  Unconventional superconductivity on a topological insulator. , 2009, Physical Review Letters.

[22]  Q. Xue,et al.  Crossover between weak antilocalization and weak localization in a magnetically doped topological insulator. , 2011, Physical review letters.

[23]  J. Smet,et al.  Tunable Surface Conductivity in Bi2Se3 Revealed in Diffusive Electron Transport , 2011, 1104.0986.

[24]  Evelyn Tang,et al.  Strain-induced partially flat band, helical snake states and interface superconductivity in topological crystalline insulators , 2014, Nature Physics.

[25]  Yanfei Zhao,et al.  Crossover from 3D to 2D quantum transport in Bi2Se3/In2Se3 superlattices. , 2014, Nano letters.

[26]  N. Peranio,et al.  Room temperature MBE deposition of Bi2Te3 and Sb2Te3 thin films with low charge carrier densities , 2012 .

[27]  J. Zhong,et al.  Anisotropic interactions and strain-induced topological phase transition in Sb2Se3 and Bi2Se3 , 2011 .

[28]  B. Iversen,et al.  Surface-dominated transport on a bulk topological insulator. , 2014, Nano letters.

[29]  R. Xiong,et al.  Low thermal conductivity and high thermoelectric figure of merit in p-type Sb2Te3/poly(3,4-ethylenedioxythiophene) thermoelectric composites , 2014 .

[30]  C. Chamon,et al.  Interaction of phonons and dirac fermions on the surface of Bi2Se3: a strong Kohn anomaly. , 2011, Physical review letters.

[31]  M. Matsunami,et al.  Fermi-Level Tuning of Topological Insulator Thin Films , 2013 .

[32]  M. Cho,et al.  Electronic structure of Te/Sb/Ge and Sb/Te/Ge multi layer films using photoelectron spectroscopy. , 2009, Journal of the American Chemical Society.

[33]  W. Duan,et al.  Design of strain-engineered quantum tunneling devices for topological surface states , 2012 .

[34]  A. Damascelli,et al.  Rashba spin-splitting control at the surface of the topological insulator Bi2Se3. , 2011, Physical review letters.

[35]  Xin Sun,et al.  Tensile strain switched ferromagnetism in layered NbS2 and NbSe2. , 2012, ACS nano.

[36]  M. Burghard,et al.  Gate-controlled linear magnetoresistance in thin Bi2Se3 sheets , 2012 .

[37]  C. Kane,et al.  Observation of Unconventional Quantum Spin Textures in Topological Insulators , 2009, Science.

[38]  Xi Dai,et al.  Topological insulators in Bi 2 Se 3 , Bi 2 Te 3 and Sb 2 Te 3 with a single Dirac cone on the surface , 2009 .

[39]  C. Kane,et al.  Theoretical Investigation of the Evolution of the Topological Phase of Bi 2 Se 3 under Mechanical Strain , 2011, 1106.5556.

[40]  M. Weinert,et al.  Tuning Dirac states by strain in the topological insulator Bi2Se3 , 2014, Nature Physics.

[41]  S. Hasegawa,et al.  In situ magnetotransport measurements in ultrathin Bi films: evidence for surface-bulk coherent transport. , 2014, Physical Review Letters.

[42]  Jung-Hyuk Koh,et al.  Effect of electronic contribution on temperature-dependent thermal transport of antimony telluride thin film , 2015 .

[43]  J. Moodera,et al.  Electrically tunable surface-to-bulk coherent coupling in topological insulator thin films , 2011, 1104.1404.

[44]  Gustav Bihlmayer,et al.  Observation of unconventional quantum spin textures in topological insulators , 2009 .

[45]  Chao Zhang,et al.  Room temperature giant and linear magnetoresistance in topological insulator Bi2Te3 nanosheets. , 2012, Physical review letters.

[46]  T. V. Ramakrishnan,et al.  Disordered electronic systems , 1985 .

[47]  M. Winterer,et al.  Strain state, film and surface morphology of epitaxial topological insulator Bi2Se3 films on Si(111) , 2014 .