Modelling Seasonal GWR of Daily PM2.5 with Proper Auxiliary Variables for the Yangtze River Delta

Over the past decades, regional haze episodes have frequently occurred in eastern China, especially in the Yangtze River Delta (YRD). Satellite derived Aerosol Optical Depth (AOD) has been used to retrieve the spatial coverage of PM2.5 concentrations. To improve the retrieval accuracy of the daily AOD-PM2.5 model, various auxiliary variables like meteorological or geographical factors have been adopted into the Geographically Weighted Regression (GWR) model. However, these variables are always arbitrarily selected without deep consideration of their potentially varying temporal or spatial contributions in the model performance. In this manuscript, we put forward an automatic procedure to select proper auxiliary variables from meteorological and geographical factors and obtain their optimal combinations to construct four seasonal GWR models. We employ two different schemes to comprehensively test the performance of our proposed GWR models: (1) comparison with other regular GWR models by varying the number of auxiliary variables; and (2) comparison with observed ground-level PM2.5 concentrations. The result shows that our GWR models of “AOD + 3” with three common meteorological variables generally perform better than all the other GWR models involved. Our models also show powerful prediction capabilities in PM2.5 concentrations with only slight overfitting. The determination coefficients R2 of our seasonal models are 0.8259 in spring, 0.7818 in summer, 0.8407 in autumn, and 0.7689 in winter. Also, the seasonal models in summer and autumn behave better than those in spring and winter. The comparison between seasonal and yearly models further validates the specific seasonal pattern of auxiliary variables of the GWR model in the YRD. We also stress the importance of key variables and propose a selection process in the AOD-PM2.5 model. Our work validates the significance of proper auxiliary variables in modelling the AOD-PM2.5 relationships and provides a good alternative in retrieving daily PM2.5 concentrations from remote sensing images in the YRD.

[1]  Zhiyong Hu,et al.  Spatial analysis of MODIS aerosol optical depth, PM2.5, and chronic coronary heart disease , 2009, International journal of health geographics.

[2]  Judith C. Chow,et al.  Impact of biomass burning on haze pollution in the Yangtze River delta, China: a case study in summer 2011 , 2013 .

[3]  W. You,et al.  Estimating ground-level PM10 concentration in northwestern China using geographically weighted regression based on satellite AOD combined with CALIPSO and MODIS fire count , 2015 .

[4]  Yang Liu,et al.  Satellite-Based Spatiotemporal Trends in PM2.5 Concentrations: China, 2004–2013 , 2015, Environmental health perspectives.

[5]  J. Schwartz,et al.  Assessing temporally and spatially resolved PM2.5 exposures for epidemiological studies using satellite aerosol optical depth measurements , 2011 .

[6]  Y-K Tu,et al.  Problems of correlations between explanatory variables in multiple regression analyses in the dental literature , 2005, British Dental Journal.

[7]  Zhengqiang Li,et al.  Remote sensing of atmospheric fine particulate matter (PM2.5) mass concentration near the ground from satellite observation , 2015 .

[8]  Jie Tian,et al.  A semi-empirical model for predicting hourly ground-level fine particulate matter (PM2.5) concentration in southern Ontario from satellite remote sensing and ground-based meteorological measurements , 2010 .

[9]  Yongming Han,et al.  Spatial and seasonal variations of PM2.5 mass and species during 2010 in Xi'an, China. , 2015, The Science of the total environment.

[10]  Yang Liu,et al.  Estimating Regional Spatial and Temporal Variability of PM2.5 Concentrations Using Satellite Data, Meteorology, and Land Use Information , 2009, Environmental health perspectives.

[11]  R. Martin,et al.  Fifteen-year global time series of satellite-derived fine particulate matter. , 2014, Environmental science & technology.

[12]  M. Charlton,et al.  Geographically Weighted Regression: A Natural Evolution of the Expansion Method for Spatial Data Analysis , 1998 .

[13]  Jan Hauke,et al.  Comparison of Values of Pearson's and Spearman's Correlation Coefficients on the Same Sets of Data , 2011 .

[14]  J. Fung,et al.  Using satellite remote sensing data to estimate the high-resolution distribution of ground-level PM2.5 , 2015 .

[15]  William L. Crosson,et al.  Estimating Ground-Level PM(sub 2.5) Concentrations in the Southeastern United States Using MAIAC AOD Retrievals and a Two-Stage Model , 2014 .

[16]  W. You,et al.  Estimating national-scale ground-level PM25 concentration in China using geographically weighted regression based on MODIS and MISR AOD , 2016, Environmental Science and Pollution Research.

[17]  Jingfeng Huang,et al.  A satellite-based geographically weighted regression model for regional PM2.5 estimation over the Pearl River Delta region in China , 2014 .

[18]  Wei Jiang,et al.  Role of bovine serum albumin and humic acid in the interaction between SiO2 nanoparticles and model cell membranes. , 2016, Environmental pollution.

[19]  Xiaoping Liu,et al.  Satellite-based ground PM 2.5 estimation using timely structure adaptive modeling , 2016 .

[20]  Lei Li,et al.  Remote sensing of atmospheric particulate mass of dry PM2.5 near the ground: Method validation using ground-based measurements , 2016 .

[21]  A. Strawa,et al.  Improving retrievals of regional fine particulate matter concentrations from Moderate Resolution Imaging Spectroradiometer (MODIS) and Ozone Monitoring Instrument (OMI) multisatellite observations , 2013, Journal of the Air & Waste Management Association.

[22]  Yang Liu,et al.  Estimating ground-level PM2.5 in China using satellite remote sensing. , 2014, Environmental science & technology.

[23]  D. Jacob,et al.  Mapping annual mean ground‐level PM2.5 concentrations using Multiangle Imaging Spectroradiometer aerosol optical thickness over the contiguous United States , 2004 .

[24]  O. Boucher,et al.  A satellite view of aerosols in the climate system , 2002, Nature.

[25]  D. Dockery,et al.  An association between air pollution and mortality in six U.S. cities. , 1993, The New England journal of medicine.

[26]  Richard T Burnett,et al.  High-Resolution Satellite-Derived PM2.5 from Optimal Estimation and Geographically Weighted Regression over North America. , 2015, Environmental science & technology.

[27]  Weiwei Sun,et al.  Investigating metrological and geographical effect in remote sensing retrival of PM2.5 concentration in Yangtze River Delta , 2016, 2016 IEEE International Geoscience and Remote Sensing Symposium (IGARSS).

[28]  Itai Kloog,et al.  Low-Concentration PM2.5 and Mortality: Estimating Acute and Chronic Effects in a Population-Based Study , 2015, Environmental health perspectives.

[29]  Scott Weichenthal,et al.  Long-Term Exposure to Fine Particulate Matter: Association with Nonaccidental and Cardiovascular Mortality in the Agricultural Health Study Cohort , 2014, Environmental health perspectives.

[30]  M. G. Estes,et al.  Estimating ground-level PM(2.5) concentrations in the southeastern U.S. using geographically weighted regression. , 2013, Environmental research.

[31]  N. Lu,et al.  Spatiotemporal distribution and short-term trends of particulate matter concentration over China, 2006–2010 , 2014, Environmental Science and Pollution Research.

[32]  Nan Li,et al.  Assessment of human exposure level to PM10 in China , 2013 .

[33]  Yuan Zhou,et al.  A Geographically and Temporally Weighted Regression Model for Ground-Level PM2.5 Estimation from Satellite-Derived 500 m Resolution AOD , 2016, Remote. Sens..

[34]  Dong Jiang,et al.  Spatio-Temporal Variation of PM2.5 Concentrations and Their Relationship with Geographic and Socioeconomic Factors in China , 2013, International journal of environmental research and public health.

[35]  Mu Qua Assessment of the Trend of Heavy PM_(2.5) Pollution Days and Economic Loss of Health Effects during 2001–2013 , 2015 .

[36]  Kebin He,et al.  Acute health impacts of airborne particles estimated from satellite remote sensing. , 2013, Environment international.

[37]  Yang Liu,et al.  Satellite-derived high resolution PM2.5 concentrations in Yangtze River Delta Region of China using improved linear mixed effects model , 2016 .

[38]  Xingfa Gu,et al.  Comparison of Four Ground-Level PM2.5 Estimation Models Using PARASOL Aerosol Optical Depth Data from China , 2016, International journal of environmental research and public health.

[39]  Yi Li,et al.  National-Scale Estimates of Ground-Level PM2.5 Concentration in China Using Geographically Weighted Regression Based on 3 km Resolution MODIS AOD , 2016, Remote. Sens..

[40]  E. Vermote,et al.  The MODIS Aerosol Algorithm, Products, and Validation , 2005 .