Aerosol properties over the western Mediterranean basin: temporal and spatial variability

Abstract. This study focuses on the analysis of Aerosol Robotic Network (AERONET) aerosol data obtained over Alboran Island (35.90° N, 3.03° W, 15 m a.s.l.) in the western Mediterranean from July 2011 to January 2012. Additional aerosol data from the three nearest AERONET stations (Malaga, Oujda and Palma de Mallorca) and the Maritime Aerosol Network (MAN) were also analyzed in order to investigate the temporal and spatial variations of aerosol over this scarcely explored region. High aerosol loads over Alboran were mainly associated with desert dust transport from North Africa and occasional advection of anthropogenic fine particles from central European urban-industrial areas. The fine particle load observed over Alboran was surprisingly similar to that obtained over the other three nearest AERONET stations, suggesting homogeneous spatial distribution of fine particle loads over the four studied sites in spite of the large differences in local sources. The results from MAN acquired over the Mediterranean Sea, Black Sea and Atlantic Ocean from July to November 2011 revealed a pronounced predominance of fine particles during the cruise period.

[1]  R. Betts,et al.  Changes in Atmospheric Constituents and in Radiative Forcing. Chapter 2 , 2007 .

[2]  F. J. Olmoa,et al.  Atmospheric aerosols during the 2003 heat wave in southeastern Spain II : Microphysical columnar properties and radiative forcing , 2006 .

[3]  F. Monteleone,et al.  Seasonal transport patterns of intense Saharan dust events at the Mediterranean island of Lampedusa , 2008 .

[4]  P. Formenti,et al.  Climatological aspects of aerosol optical properties in Northern Greece , 2003 .

[5]  V. Masson,et al.  Satellite climatology of African dust transport in the Mediterranean atmosphere , 1998 .

[6]  L. Alados-Arboledas,et al.  Global and diffuse shortwave irradiance during a strong desert dust episode at Granada (Spain) , 2012 .

[7]  S. Solomon The Physical Science Basis : Contribution of Working Group I to the Fourth Assessment Report of the Intergovernmental Panel on Climate Change , 2007 .

[8]  María P. Utrillas,et al.  Columnar aerosol properties in Valencia (Spain) by ground‐based Sun photometry , 2007 .

[9]  Alexander Smirnov,et al.  Maritime Aerosol Network as a component of Aerosol Robotic Network , 2009 .

[10]  Lucas Alados-Arboledas,et al.  Aerosol radiative forcing during African desert dust events (2005–2010) over Southeastern Spain , 2012 .

[11]  Didier Tanré,et al.  Remote sensing of aerosols over the oceans using MSG/SEVIRI imagery , 2005 .

[12]  G. Sumner,et al.  Precipitation seasonality in eastern and southern coastal Spain , 2001 .

[13]  O. Boucher,et al.  Estimates of the direct and indirect radiative forcing due to tropospheric aerosols: A review , 2000 .

[14]  Daniela Meloni,et al.  Aerosol optical properties at Lampedusa (Central Mediterranean). 1. Influence of transport and identification of different aerosol types , 2005 .

[15]  L. Alados-Arboledas,et al.  Optical and microphysical properties of fresh biomass burning aerosol retrieved by Raman lidar, and star‐and sun‐photometry , 2011 .

[16]  Gionata Biavati,et al.  Seasonal behavior of Saharan dust events at the Mediterranean island of Lampedusa in the period 1999-2005 , 2007 .

[17]  D. Meloni,et al.  Large atmospheric shortwave radiative forcing by Mediterranean aerosols derived from simultaneous ground‐based and spaceborne observations and dependence on the aerosol type and single scattering albedo , 2010 .

[18]  Victoria E. Cachorro,et al.  Aerosol optical depth and Ångström exponent climatology at El Arenosillo AERONET site (Huelva, Spain) , 2007 .

[19]  T. Eck,et al.  Optical Properties of Atmospheric Aerosol in Maritime Environments , 2002 .

[20]  H. Sauerzopf,et al.  Optical characteristics of the aerosol in Spain and Austria and its effect on radiative forcing , 2002 .

[21]  Robert Frouin,et al.  Maritime aerosol optical thickness measured by handheld sun photometers , 2004 .

[22]  L. Alados-Arboledas,et al.  Classification of aerosol radiative properties during African desert dust intrusions over southeastern Spain by sector origins and cluster analysis , 2012 .

[23]  Lorraine Remer,et al.  The MODIS 2.1-μm channel-correlation with visible reflectance for use in remote sensing of aerosol , 1997, IEEE Trans. Geosci. Remote. Sens..

[24]  L. Alados-Arboledas,et al.  Aerosol size properties at Armilla, Granada (Spain) , 2003 .

[25]  P. Crutzen,et al.  Absorbing mediterranean aerosols lead to a large reduction in the solar radiation at the surface , 2002 .

[26]  M. P. Utrillas,et al.  Evaluation of the new ESR network software for the retrieval of direct sun products from CIMEL CE318 and PREDE POM01 sun-sky radiometers , 2012 .

[27]  Ilan Koren,et al.  The effect of smoke, dust, and pollution aerosol on shallow cloud development over the Atlantic Ocean. , 2005, Proceedings of the National Academy of Sciences of the United States of America.

[28]  J. Lelieveld,et al.  Global Air Pollution Crossroads over the Mediterranean , 2002, Science.

[29]  Daniela Meloni,et al.  Forest fire aerosol over the Mediterranean basin during summer 2003 , 2005 .

[30]  B. Langmann,et al.  Impact of ship emissions on the Mediterranean summertime pollution and climate: A regional model study , 2005 .

[31]  Alexander Smirnov,et al.  Maritime component in aerosol optical models derived from Aerosol Robotic Network data , 2003 .

[32]  Alexander Smirnov,et al.  A Pure Marine Aerosol Model, for Use in Remote Sensing Applications , 2012 .

[33]  F. Monteleone,et al.  Surface shortwave radiative forcing of different aerosol types in the central Mediterranean , 2008 .

[34]  Christos Matsoukas,et al.  The direct effect of aerosols on solar radiation over the broader Mediterranean basin , 2011 .

[35]  Giorgio Fiocco,et al.  Tropospheric aerosols in the Mediterranean: 1. Microphysical and optical properties , 2003 .

[36]  Mar Viana,et al.  Chemical tracers of particulate emissions from commercial shipping. , 2009, Environmental science & technology.

[37]  Alexander Smirnov,et al.  Maritime aerosol network as a component of AERONET - first results and comparison with global aerosol models and satellite retrievals , 2011 .

[38]  T. Eck,et al.  Variability of Absorption and Optical Properties of Key Aerosol Types Observed in Worldwide Locations , 2002 .

[39]  R. Draxler HYSPLIT (HYbrid Single-Particle Lagrangian Integrated Trajectory) Model access via NOAA ARL READY Website , 2010 .

[40]  L. Alados-Arboledas,et al.  Columnar aerosol properties from sun-and-star photometry: statistical comparisons and day-to-night dynamic , 2012 .

[41]  J. Haywood,et al.  Multi‐spectral calculations of the direct radiative forcing of tropospheric sulphate and soot aerosols using a column model , 1997 .

[42]  Jean-Claude Roger,et al.  One year measurements of aerosol optical properties over an urban coastal site: Effect on local direct radiative forcing , 2008 .

[43]  Franco Lucarelli,et al.  Evidence for heavy fuel oil combustion aerosols from chemical analyses at the island of Lampedusa: a possible large role of ships emissions in the Mediterranean , 2012 .

[44]  Oleg Dubovik,et al.  Microphysical and optical properties of aerosol particles in urban zone during ESCOMPTE , 2003 .

[45]  G. Gobbi,et al.  Aerosol seasonal variability over the Mediterranean region and relative impact of maritime, continental and Saharan dust particles over the basin from MODIS data in the year 2001 , 2004 .

[46]  Xavier Querol,et al.  Spatial and temporal variability in aerosol properties over the Mediterranean basin based on 6-year (2000-2006) MODIS data , 2008 .

[47]  L. Mona,et al.  Multi year sun-photometer measurements for aerosol characterization in a Central Mediterranean site , 2012 .

[48]  D. Hatzidimitriou,et al.  Aerosol physical and optical properties in the Eastern Mediterranean Basin, Crete, from Aerosol Robotic Network data , 2006 .

[49]  X. Querol,et al.  Source apportionment of PM10 and PM2.5 at multiple sites in the strait of Gibraltar by PMF: impact of shipping emissions , 2011, Environmental science and pollution research international.

[50]  B. Holben,et al.  Estimating Marine Aerosol Particle Volume and Number from Maritime Aerosol Network Data , 2012 .

[51]  T. Cokacar,et al.  Optical properties of mineral dust outbreaks over the northeastern Mediterranean , 2003 .

[52]  A. Alcantara,et al.  Atmospheric aerosols during the 2003 heat wave in southeastern Spain I: Spectral optical depth , 2006 .

[53]  Christos Zerefos,et al.  Aerosol optical properties and large‐scale transport of air masses: Observations at a coastal and a semiarid site in the eastern Mediterranean during summer 1998 , 2001 .

[54]  George Kallos,et al.  Photooxidant dynamics in the Mediterranean basin in summer: Results from European research projects , 1997 .

[55]  Lucas Alados-Arboledas,et al.  Saharan dust outbreak over southeastern Spain as detected by sun photometer , 2005 .

[56]  A. Smirnov,et al.  AERONET-a federated instrument network and data archive for aerosol Characterization , 1998 .

[57]  C. Zerefos,et al.  Raman lidar and sunphotometric measurements of aerosol optical properties over Thessaloniki, Greece during a biomass burning episode , 2003 .

[58]  R. Kahn,et al.  Absorption properties of Mediterranean aerosols obtained from multi-year ground-based remote sensing observations , 2013 .

[59]  L. Alados-Arboledas,et al.  Estimating aerosol characteristics from solar irradiance measurements at an urban location in southeastern Spain , 2014 .

[60]  T. Eck,et al.  Spectral discrimination of coarse and fine mode optical depth , 2003 .