Absorption effects on microdroplet resonant emission structure.

The effect of absorption on microdroplet resonance emission line intensities was studied in 15-microm-diameter Rhodamine 6G/ethanol solution droplets. Absorption was controlled by varying the concentration of the additive nigrosin. Spectrally integrated intensities of resonant features are found to be proportional to a droplet cavity mode efficiency Q(a)/(Q(a)+Q(o)) expressed in terms of cavity output coupling and absorption factors Q(o) and Q(a), respectively. These Q's are determined from linewidths calculated from Lorenz-Mie theory by using combinations of the real and complex indices of refraction. An experimental upper limit of Q for first-order modes was determined to be 10(8) from the data.

[1]  C K Rushforth,et al.  Sizing dielectric spheres and cylinders by aligning measured and computed resonance locations: algorithm for multiple orders. , 1985, Applied optics.

[2]  R. Chang,et al.  Laser emission from individual droplets at wavelengths corresponding to morphology-dependent resonances. , 1984, Optics letters.

[3]  A. Campillo,et al.  Vibrating orifice droplet generator for precision optical studies , 1990 .

[4]  A. Campillo,et al.  Double-resonance stimulated Raman scattering in micrometer-sized droplets , 1990 .

[5]  P. Chylek Partial-wave resonances and the ripple structure in the Mie normalized extinction cross section , 1976 .

[6]  Lin,et al.  Cavity quantum electrodynamic enhancement of stimulated emission in microdroplets. , 1991, Physical review letters.

[7]  S. C. Hill,et al.  Morphology-dependent resonances associated with stimulated processes in microspheres , 1986, International Laser Science Conference.

[8]  Robert E. Benner,et al.  Observation of Structure Resonances in the Fluorescence Spectra from Microspheres , 1980 .

[9]  Jeffrey T. Kiehl,et al.  Optical levitation and partial-wave resonances , 1978 .

[10]  Alan L. Huston,et al.  Spherical-cavity-mode assignments of optical resonances in microdroplets using elastic scattering , 1990 .

[11]  A. Campillo,et al.  Nonlinear Mie scattering: electrostrictive coupling of light to droplet acoustic modes. , 1990, Optics Letters.

[12]  R. G. Pinnick,et al.  Time-resolved spectroscopy of laser emission from dye-doped droplets. , 1989, Optics letters.

[13]  Chew Radiation and lifetimes of atoms inside dielectric particles. , 1988, Physical review. A, General physics.

[14]  H. M. Lai,et al.  Dielectric microspheres as optical cavities: thermal spectrum and density of states , 1987 .