Long-term variation of black carbon and PM2.5 in Beijing, China with respect to meteorological conditions and governmental measures.

Black carbon (BC) and PM2.5 were studied for nine years from 2005 to 2013 in the Beijing urban area. The overall weekly average mass concentrations of BC and PM2.5 were 4.3 and 66.8 μg/m³. PM2.5 annual means of the nine years are around 2 times of the standard (GB3095-2012) in China, and are 5-7 times higher than the WHO standard. The Beijing Olympic Games in 2008 was a milestone to mitigate aerosol pollution. Temporal distribution of BC shows a distinct declining trend, and annual mean mass concentrations of PM2.5 after 2008 were lower than those before 2008 but increased from 2011 to 2013. Wind rose plots show that high BC concentrations are usually associated with low wind speed of northeastern or southwestern winds, generally causing poor visibility. Governmental mitigation measures such as traffic restriction despite increased motor vehicle numbers and gasoline consumption and industry relocation with declining consumption of coal and coke were successful in reducing BC emissions. Annual mean of BC was reduced by 38% in 2013 compared to 2005. However, BC contamination in Beijing is still severe when compared to other urban areas around the world.

[1]  K. Straif,et al.  Exposure to nitrosamines, carbon black, asbestos, and talc and mortality from stomach, lung, and laryngeal cancer in a cohort of rubber workers. , 2000, American journal of epidemiology.

[2]  J. Hansen,et al.  Climate Effects of Black Carbon Aerosols in China and India , 2002, Science.

[3]  J. Hansen,et al.  Global warming in the twenty-first century: an alternative scenario. , 2000, Proceedings of the National Academy of Sciences of the United States of America.

[4]  R. Hitzenberger,et al.  Development of an improved optical transmission technique for black carbon (BC) analysis , 2001 .

[5]  A. S. Emilenko,et al.  Black carbon particles in the urban atmosphere in Beijing , 2005 .

[6]  Kebin He,et al.  The characteristics of PM2.5 in Beijing, China , 2001 .

[7]  Peter Wåhlin,et al.  A European aerosol phenomenology—1: physical characteristics of particulate matter at kerbside, urban, rural and background sites in Europe , 2004 .

[8]  Jiming Hao,et al.  Black carbon at a roadside site in Beijing: Temporal variations and relationships with carbon monoxide and particle number size distribution , 2013 .

[9]  H. Akimoto,et al.  Mass concentrations of black carbon measured by four instruments in the middle of Central East China in June 2006 , 2008 .

[10]  Yang Yu,et al.  Dynamics and origin of PM2.5 during a three-year sampling period in Beijing, China. , 2011, Journal of environmental monitoring : JEM.

[11]  M. Jacobson,et al.  Strong radiative heating due to the mixing state of black carbon in atmospheric aerosols , 2022 .

[12]  D. Streets,et al.  A technology‐based global inventory of black and organic carbon emissions from combustion , 2004 .

[13]  G. Wolff Particulate Elemental Carbon in the Atmosphere , 1981 .

[14]  Chang-hong Chen,et al.  Concentrations, seasonal and diurnal variations of black carbon in PM2.5 in Shanghai, China , 2014 .

[15]  Ruizhong Rao,et al.  Black carbon aerosols in urban central China , 2015 .

[16]  J. Kahl,et al.  20th-Century Industrial Black Carbon Emissions Altered Arctic Climate Forcing , 2007, Science.

[17]  Xiaohui Xu,et al.  Differentiating the associations of black carbon and fine particle with daily mortality in a Chinese city. , 2013, Environmental research.

[18]  J. Heintzenberg Size-segregated measurements of particulate elemental carbon and aerosol light absorption at remote arctic locations , 1982 .

[19]  Michael Q. Wang,et al.  Black carbon emissions in China , 2001 .

[20]  G. Carmichael,et al.  Asian emissions in 2006 for the NASA INTEX-B mission , 2009 .

[21]  P. S. Praveen,et al.  Seasonal variation of black carbon aerosols over a tropical urban city of Pune, India , 2007 .

[22]  A. Petzold,et al.  Intercomparison of thermal and optical measurement methods for elemental carbon and black carbon at an urban location. , 2006, Environmental science & technology.

[23]  S. C. Liu,et al.  Case study of the effects of atmospheric aerosols and regional haze on agriculture: an opportunity to enhance crop yields in China through emission controls? , 1999, Proceedings of the National Academy of Sciences of the United States of America.

[24]  Mao Jietai,et al.  Observation of black carbon aerosol in Beijing, 2003 , 2007 .

[25]  Yuan Chen,et al.  The Effect of Government Policies on the Temporal Development of Contamination Characteristics Within the Aerosol Distribution in Beijing, China , 2013 .

[26]  K. Cen,et al.  A review on black carbon emissions, worldwide and in China. , 2014, Chemosphere.

[27]  D. Koch,et al.  Quantifying immediate radiative forcing by black carbon and organic matter with the Specific Forcing Pulse , 2010 .

[28]  Chen Zonglian,et al.  Measurement and Analysis for Atmospheric Aerosol Particulates in Beijing , 1994 .

[29]  P. Hopke,et al.  Characteristics of the major chemical constituents of PM2.5 and smog events in Seoul, Korea in 2003 and 2004 , 2007 .

[30]  M. Bergin,et al.  Soot Takes Center Stage , 2002, Science.

[31]  Qiang Zhang,et al.  Sulfur dioxide and primary carbonaceous aerosol emissions in China and India, 1996-2010 , 2011 .

[32]  Jiming Hao,et al.  Evaluating the air quality impacts of the 2008 Beijing Olympic Games: On-road emission factors and black carbon profiles , 2009 .

[33]  Tong Yu,et al.  Identification and estimate of biomass burning contribution to the urban aerosol organic carbon concentrations in Beijing , 2004 .

[34]  R. Hillamo,et al.  Atmospheric black carbon in Helsinki , 1998 .

[35]  P. Zhao,et al.  Characteristics of carbonaceous aerosol in the region of Beijing, Tianjin, and Hebei, China , 2013 .

[36]  H. Cachier,et al.  Beijing aerosol: Atmospheric interactions and new trends , 2007 .

[37]  J. Chow,et al.  Black carbon relationships with emissions and meteorology in Xi'an, China , 2009 .

[38]  L. Alados-Arboledas,et al.  Black carbon aerosols over an urban area in south-eastern Spain: Changes detected after the 2008 economic crisis , 2011 .

[39]  Judith C. Chow,et al.  Comparison and evaluation of in situ and filter carbon measurements at the Fresno Supersite , 2002 .

[40]  U. Kaminski,et al.  Spatio-temporal variations of black carbon concentrations in the Megacity Beijing. , 2013, Environmental pollution.

[41]  J. Penner,et al.  Carbonaceous particles in the atmosphere: A historical perspective to the Fifth International Conference on Carbonaceous Particles in the Atmosphere , 1996 .

[42]  Stefan Norra,et al.  Efficiency of mitigation measures to reduce particulate air pollution--a case study during the Olympic Summer Games 2008 in Beijing, China. , 2012, The Science of the total environment.

[43]  J. Chow,et al.  Variability of organic and elemental carbon, water soluble organic carbon, and isotopes in Hong Kong , 2006 .

[44]  Hairong Tao,et al.  The characteristics of carbonaceous species and their sources in PM2.5 in Beijing , 2004 .

[45]  Yuan Chen,et al.  The influence of governmental mitigation measures on contamination characteristics of PM(2.5) in Beijing. , 2014, The Science of the total environment.

[46]  G. Cao,et al.  Inventory of black carbon and organic carbon emissions from China , 2006 .

[47]  V. Ramanathan,et al.  Global and regional climate changes due to black carbon , 2008 .

[48]  Herek L. Clack,et al.  Particulate carbon emissions from ESPs during injection of powdered mercury sorbents: Updated estimates based on the U.S. EPA report to congress on black carbon , 2012 .

[49]  H. Akimoto,et al.  An Asian emission inventory of anthropogenic emission sources for the period 1980-2020 , 2007 .

[50]  N. Takegawa,et al.  Reduction of black carbon aerosols in Tokyo: Comparison of real-time observations with emission estimates , 2012 .

[51]  H. R. Anderson,et al.  Black Carbon as an Additional Indicator of the Adverse Health Effects of Airborne Particles Compared with PM10 and PM2.5 , 2011, Environmental health perspectives.

[52]  J. Chow,et al.  Carbonaceous and Ionic Components of Atmospheric Fine Particles in Beijing and Their Impact on Atmospheric Visibility , 2012 .

[53]  Jiming Hao,et al.  Quantifying the air pollutants emission reduction during the 2008 Olympic games in Beijing. , 2010, Environmental science & technology.

[54]  M. Lippmann,et al.  Associations between Health Effects and Particulate Matter and Black Carbon in Subjects with Respiratory Disease , 2005, Environmental health perspectives.

[55]  Judith C. Chow,et al.  Characteristics of carbonaceous aerosol in Pearl River Delta Region, China during 2001 winter period , 2003 .

[56]  V. Dietze,et al.  The effect of mitigation measures on size distributed mass concentrations of atmospheric particles and black carbon concentrations during the Olympic Summer Games 2008 in Beijing. , 2011, The Science of the total environment.