Spontaneous current constriction in threshold switching devices

Threshold switching devices are of increasing importance for a number of applications including solid-state memories and neuromorphic circuits. Their non-linear characteristics are thought to be associated with a spontaneous (occurring without an apparent external stimulus) current flow constriction but the extent and the underlying mechanism are a subject of debate. Here we use Scanning Joule Expansion Microscopy to demonstrate that, in functional layers with thermally activated electrical conductivity, the current spontaneously and gradually constricts when a device is biased into the negative differential resistance region. We also show that the S-type negative differential resistance I–V characteristics are only a subset of possible solutions and it is possible to have multiple current density distributions corresponding to the same value of the device voltage. In materials with steep dependence of current on temperature the current constriction can occur in nanoscale devices, making this effect relevant for computing applications.Today the phenomenon underlying threshold switching of Oxide-based resistive memories is an unresolved debate. Here, the authors report that the TaOx-based conductive filament formation, the current density and temperature are not-uniform distributions and electric field domains are not required.

[1]  J. Bain,et al.  Electronic Instabilities Leading to Electroformation of Binary Metal Oxide‐based Resistive Switches , 2014 .

[2]  Marek Skowronski,et al.  Electro-Thermal Model of Threshold Switching in TaOx-Based Devices. , 2017, ACS applied materials & interfaces.

[3]  Matthew D. Pickett,et al.  Local Temperature Redistribution and Structural Transition During Joule‐Heating‐Driven Conductance Switching in VO2 , 2013, Advanced materials.

[4]  R. Williams,et al.  Separation of current density and electric field domains caused by nonlinear electronic instabilities , 2018, Nature Communications.

[5]  R. Stanley Williams,et al.  An accurate locally active memristor model for S-type negative differential resistance in NbOx , 2016 .

[6]  Ronald Tetzlaff,et al.  Physical model of threshold switching in NbO2 based memristors , 2015 .

[7]  Marek Skowronski,et al.  Formation of the Conducting Filament in TaO x-Resistive Switching Devices by Thermal-Gradient-Induced Cation Accumulation. , 2018, ACS applied materials & interfaces.

[8]  Fan Yang,et al.  Anomalously low electronic thermal conductivity in metallic vanadium dioxide , 2017, Science.

[9]  Rainer Waser,et al.  Multidimensional Simulation of Threshold Switching in NbO2 Based on an Electric Field Triggered Thermal Runaway Model , 2016 .

[10]  Jonathan M. Goodwill,et al.  ON-state evolution in lateral and vertical VO2 threshold switching devices , 2017, Nanotechnology.

[11]  Jonathan M. Goodwill,et al.  Scaling behavior of oxide-based electrothermal threshold switching devices. , 2017, Nanoscale.

[12]  R. Waser,et al.  Thermochemical resistive switching: materials, mechanisms, and scaling projections , 2011 .

[13]  James A. Bain,et al.  High-Frequency TaOx-Based Compact Oscillators , 2015, IEEE Transactions on Electron Devices.

[14]  A. Majumdar,et al.  Scanning Joule expansion microscopy at nanometer scales , 1998 .

[15]  E. J. Rymaszewski,et al.  Dielectric constant dependence of Poole-Frenkel potential in tantalum oxide thin films , 1994 .

[16]  Rolf Landauer,et al.  Electrical conductivity in inhomogeneous media , 2008 .

[17]  T. Tseng,et al.  Conduction mechanisms in amorphous and crystalline Ta2O5 thin films , 1998 .

[18]  James A. Bain,et al.  Switching dynamics of TaOx-based threshold switching devices , 2018 .

[19]  P. Narayanan,et al.  Access devices for 3D crosspoint memorya) , 2014 .

[20]  D. Strukov,et al.  Thermophoresis/diffusion as a plausible mechanism for unipolar resistive switching in metal–oxide–metal memristors , 2012, Applied Physics A.

[21]  J. Frenkel,et al.  On Pre-Breakdown Phenomena in Insulators and Electronic Semi-Conductors , 1938 .

[22]  M Jurczak,et al.  Switching mechanism in two-terminal vanadium dioxide devices , 2015, Nanotechnology.

[23]  B. Ridley,et al.  Specific Negative Resistance in Solids , 1963 .

[24]  Z. Cen,et al.  Temperature effect on titanium nitride nanometer thin film in air , 2017 .