论文信息 - Exploring Higher-Lying Electronic States of a Molecular Switch by Coherent Triggered-Exchange 2D Electronic Spectroscopy

Exploring Higher-Lying Electronic States of a Molecular Switch by Coherent Triggered-Exchange 2D Electronic Spectroscopy

We use pump-repump-probe transient absorption spectroscopy to investigate the role of higher-lying electronic states in the photochemistry of a molecular switch. Moreover, replacing the pump pulse by a pulse-shaper-generated phase-stable double pulse, triggered-exchange two-dimensional (TE2D) electronic spectroscopy is established in the visible regime.

T. Brixner | J. Buback | P. Nuernberger | Martin Kullmann | Stefan Ruetzel

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