Effect of intense chirped pulses on the coherent phonon generation in Te

The authors have studied the influence of chirped laser pulses on the coherent phonon generation in single crystal Te. They have shown that the pulse chirp affects the amplitude of coherent phonons with A1 symmetry in the case of intense excitation only. By varying the chirp of an intense exciting pulse, the authors demonstrated that negatively chirped pulses are almost twice more effective in the creation of lattice coherence than positively chirped pulses.

[1]  T. Dekorsy,et al.  Observation of longitudinal optical–transverse optical splitting for E-symmetry phonons in Te by coherent phonon spectroscopy , 2005 .

[2]  C. Roeser,et al.  Optical control of coherent lattice vibrations in tellurium , 2004 .

[3]  S. Fahy,et al.  Density-functional theory approach to ultrafast laser excitation of semiconductors: Application to the A 1 phonon in tellurium , 2002 .

[4]  O. Misochko Coherent phonons and their properties , 2001 .

[5]  Roberto Merlin,et al.  Generating coherent THz phonons with light pulses , 1997 .

[6]  E. Hiller,et al.  Can chirp enhance cumulative pre‐resonant impulsive stimulated Raman excitation? , 1996 .

[7]  C. Shank,et al.  Selective excitation of vibrational wave packet motion using chirped pulses. , 1995, Physical review letters.

[8]  Kurz,et al.  Impulsive Softening of Coherent Phonons in Tellurium. , 1995, Physical review letters.

[9]  Yakovlev,et al.  Quantum Control of Wave Packet Evolution with Tailored Femtosecond Pulses. , 1995, Physical review letters.

[10]  E. Ippen,et al.  Mechanism for displacive excitation of coherent phonons in Sb, Bi, Te, and Ti2O3 , 1991 .

[11]  Stuart A. Rice,et al.  Control of selectivity of chemical reaction via control of wave packet evolution , 1985 .

[12]  H. Jerrard Light Scattering in Solids , 1972 .

[13]  G. Dresselhaus,et al.  Raman Spectra and Lattice Dynamics of Tellurium , 1971 .

[14]  K. Nelson,et al.  Time-resolved vibrational spectroscopy in the impulsive limit , 1994 .

[15]  Cheng,et al.  Theory for displacive excitation of coherent phonons. , 1992, Physical review. B, Condensed matter.