Order of Magnitude Smaller Limit on the Electric Dipole Moment of the Electron

Stubbornly Spherical The shape of the electron's charge distribution reflects the degree to which switching the direction of time impacts the basic ingredients of the universe. The Standard Model (SM) of particle physics predicts a very slight asphericity of the charge distribution, whereas SM extensions such as supersymmetry posit bigger and potentially measurable, but still tiny, deviations from a perfect sphere. Polar molecules have been identified as ideal settings for measuring this asymmetry, which should be reflected in a finite electric dipole moment (EDM) because of the extremely large effective electric fields that act on an electron inside such molecules. Using electron spin precession in the molecule ThO, Baron et al. (p. 269, published online 19 December; see the cover; see the Perspective by Brown) measured the EDM of the electron as consistent with zero. This excludes some of the extensions to the SM and sets a bound to the search for a nonzero EDM in other facilities, such as the Large Hadron Collider. Spin precession measurements in the polar molecule thorium monoxide indicate a nearly spherical charge distribution of an electron. [Also see Perspective by Brown] The Standard Model of particle physics is known to be incomplete. Extensions to the Standard Model, such as weak-scale supersymmetry, posit the existence of new particles and interactions that are asymmetric under time reversal (T) and nearly always predict a small yet potentially measurable electron electric dipole moment (EDM), de, in the range of 10−27 to 10−30 e·cm. The EDM is an asymmetric charge distribution along the electron spin (S→) that is also asymmetric under T. Using the polar molecule thorium monoxide, we measured de = (–2.1 ± 3.7stat ± 2.5syst) × 10−29 e·cm. This corresponds to an upper limit of | de | < 8.7 × 10−29 e·cm with 90% confidence, an order of magnitude improvement in sensitivity relative to the previous best limit. Our result constrains T-violating physics at the TeV energy scale.

[1]  P. Corkum,et al.  Journal of Physics B: atomic, molecular and optical physics , 2015 .

[2]  Yang Yang,et al.  Single-Crystal Linear Polymers Through Visible Light–Triggered Topochemical Quantitative Polymerization , 2014, Science.

[3]  J. Zupan,et al.  Low energy probes of PeV scale sfermions , 2013, Journal of High Energy Physics.

[4]  A. Titov,et al.  Communication: theoretical study of ThO for the electron electric dipole moment search. , 2013, The Journal of chemical physics.

[5]  P. Hess,et al.  Advanced cold molecule electron EDM , 2013, 1307.1657.

[6]  P. Hess,et al.  Shot-noise-limited spin measurements in a pulsed molecular beam , 2013, 1305.2179.

[7]  Kathy P. Wheeler,et al.  Reviews of Modern Physics , 2013 .

[8]  S. Eckel,et al.  Search for the electron electric dipole moment using $\Omega$-doublet levels in PbO$^*$ , 2013, 1303.3075.

[9]  U. van Kolck,et al.  Electric Dipole Moments of Nucleons, Nuclei, and Atoms: The Standard Model and Beyond , 2013, 1303.2371.

[10]  E. Hinds,et al.  Measurement of the electron's electric dipole moment using YbF molecules: methods and data analysis , 2012, 1208.4507.

[11]  J. Doyle,et al.  The buffer gas beam: an intense, cold, and slow source for atoms and molecules. , 2011, Chemical reviews.

[12]  V. Dzuba,et al.  Relations between matrix elements of different weak interactions and interpretation of the PNC and EDM measurements in atoms and molecules , 2011, 1109.6082.

[13]  V. Dzuba,et al.  Relations between matrix elements of different weak interactions and interpretation of the parity-nonconserving and electron electric-dipole-moment measurements in atoms and molecules , 2011 .

[14]  G. Gabrielse,et al.  Magnetic and Electric Dipole Moments of the \(H\ ^3\Delta_1\) State in ThO , 2011, 1107.2287.

[15]  E. Hinds,et al.  Improved measurement of the shape of the electron , 2011, Nature.

[16]  P. Hess,et al.  A cryogenic beam of refractory, chemically reactive molecules with expansion cooling. , 2011, Physical chemistry chemical physics : PCCP.

[17]  G. Gabrielse,et al.  Magnetic and electric dipole moments of the H3#1 state in ThO , 2011 .

[18]  Nasser Kalantar-Nayestanaki,et al.  EPJ Web of Conferences , 2010 .

[19]  P. Hamilton Preliminary results in the search for the electron electric dipole moment in PbO , 2010 .

[20]  Georg G. Raffelt,et al.  Progress in Particle and Nuclear Physics , 2010 .

[21]  G. Gabrielse,et al.  Search for the electric dipole moment of the electron with thorium monoxide , 2009, 0908.2412.

[22]  W C Griffith,et al.  Improved limit on the permanent electric dipole moment of 199Hg. , 2009, Physical review letters.

[23]  D. DeMille,et al.  Preparation and detection of states with simultaneous spin alignment and selectable molecular orientation in PbO , 2008, 0807.4851.

[24]  B. Roberts Lepton Dipole Moments , 2003, hep-ex/0309010.

[25]  E. Meyer,et al.  Prospects for an electron electric-dipole moment search in metastable ThO and ThF+ , 2008, 0805.0161.

[26]  New Journal of Physics The , 2007 .

[27]  R. Decarvalho,et al.  High-flux beam source for cold, slow atoms or molecules. , 2005, Physical review letters.

[28]  M. Pospelov,et al.  Electric dipole moments as probes of new physics , 2005, hep-ph/0504231.

[29]  John Ellis,et al.  Int. J. Mod. Phys. , 2005 .

[30]  S. Mahulikar,et al.  Physica Scripta , 2004 .

[31]  P. Malmqvist,et al.  Relativistic and correlated calculations on the ground and excited states of ThO , 2003 .

[32]  George W. Collins,et al.  Methods and Data Analysis , 2003 .

[33]  岩澤 康裕,et al.  Physical Chemistry Chemical Physics : PCCP , 2002 .

[34]  E. Commins,et al.  New limit on the electron electric dipole moment. , 2002, Physical review letters.

[35]  S. Barr,et al.  The Search for a Permanent Electric Dipole Moment , 2003 .

[36]  Feng-Lei Hong,et al.  Stabilization and frequency measurement of the I2-stabilized Nd: YAG laser , 1998, IEEE Trans. Instrum. Meas..

[37]  R. Cousins,et al.  A Unified Approach to the Classical Statistical Analysis of Small Signals , 1997, physics/9711021.

[38]  I. Khriplovich,et al.  Cp Violation Without Strangeness , 1997 .

[39]  M. Kozlov,et al.  Parity violation effects in diatomics , 1995 .

[40]  Mordechai Lando,et al.  Thermally induced window birefringence in high-power copper vapor laser , 1993, Other Conferences.

[41]  S. Barr A Review of CP violation in atoms , 1993 .

[42]  W. Bernreuther,et al.  The electric dipole moment of the electron , 1991 .

[43]  G. Edvinsson,et al.  Two new band systems in ThO , 1990 .

[44]  P. Langacker The standard model and beyond , 2009 .

[45]  C. R. Stroud,et al.  Coherent trapping of atomic populations. , 1978, Optics letters.

[46]  G Gabrielse,et al.  Measurement of the Stokes parameters of light. , 1977, Applied optics.

[47]  R A Patten Michelson interferometer as a remote gauge. , 1971, Applied optics.

[48]  M. Player,et al.  An experiment to search for an electric dipole moment in the 3P2 metastable state of xenon , 1970 .

[49]  J. C. Bevington,et al.  Chemical Reviews , 1970, Nature.

[50]  M. Gell-Mann,et al.  Physics Today. , 1966, Applied optics.

[51]  P. Sandars The electric dipole moment of an atom , 1965 .

[52]  Physical Review , 1965, Nature.

[53]  Physics Letters , 1962, Nature.

[54]  E. Parzen Annals of Mathematical Statistics , 1962 .

[55]  J. H. Curtiss,et al.  On the Distribution of the Quotient of Two Chance Variables , 1941 .

[56]  A. Hall Applied Optics. , 2022, Science.

[57]  October I Physical Review Letters , 2022 .