Measuring Trace Gas Emission from Multi-Distributed Sources Using Vertical Radial Plume Mapping (VRPM) and Backward Lagrangian Stochastic (bLS) Techniques

Two micrometeorological techniques for measuring trace gas emission rates from distributed area sources were evaluated using a variety of synthetic area sources. The vertical radial plume mapping (VRPM) and the backward Lagrangian stochastic (bLS) techniques with an open-path optical spectroscopic sensor were evaluated for relative accuracy for multiple emission-source and sensor configurations. The relative accuracy was calculated by dividing the measured emission rate by the actual emission rate; thus, a relative accuracy of 1.0 represents a perfect measure. For a single area emission source, the VRPM technique yielded a somewhat high relative accuracy of 1.38 ± 0.28. The bLS technique resulted in a relative accuracy close to unity, 0.98 ± 0.24. Relative accuracies for dual source emissions for the VRPM and bLS techniques were somewhat similar to single source emissions, 1.23 ± 0.17 and 0.94 ± 0.24, respectively. When the bLS technique was used with vertical point concentrations, the relative accuracy was unacceptably low.

[1]  R. Desjardins,et al.  Methane and ammonia emissions from a beef feedlot in western Canada for a twelve-day period in the fall , 2008 .

[2]  R. Desjardins,et al.  Multi-Source Emission Determination Using an Inverse-Dispersion Technique , 2009 .

[3]  Lowry A. Harper,et al.  Estimating gas emissions from a farm with an inverse-dispersion technique , 2005 .

[4]  R. Desjardins,et al.  Assessment of the uncertainty of using an inverse-dispersion technique to measure methane emissions from animals in a barn and in a small pen , 2010 .

[5]  Susan A. Thorneloe,et al.  Open-Path Tunable Diode Laser Absorption Spectroscopy for Acquisition of Fugitive Emission Flux Data , 2005, Journal of the Air & Waste Management Association.

[6]  Thomas K. Flesch,et al.  Ammonia emission from dairy cow manure stored in a lagoon over summer , 2008 .

[7]  T. Flesch,et al.  An approach for measuring methane emissions from whole farms. , 2006, Journal of environmental quality.

[8]  M. Sanz,et al.  Use of an inverse dispersion technique for estimating ammonia emission from surface-applied slurry. , 2010 .

[9]  Ram A. Hashmonay,et al.  Development of EPA OTM 10 for Landfill Applications , 2010 .

[10]  D. F. Natschke,et al.  Field evaluation of a method for estimating gaseous fluxes from area sources using open-path Fourier transform infrared. , 2001, Environmental science & technology.

[11]  T. Flesch,et al.  Ammonia emissions from dairy production in Wisconsin. , 2009, Journal of dairy science.

[12]  Lowry A. Harper,et al.  Deducing Ground-to-Air Emissions from Observed Trace Gas Concentrations: A Field Trial with Wind Disturbance , 2004 .

[13]  F. Kelliher,et al.  Methane emissions from dairy cows: Comparing open-path laser measurements to profile-based techniques , 2005 .

[14]  John D. Wilson,et al.  Influence of source–sensor geometry on multi-source emission rate estimates , 2008 .

[15]  Ram A Hashmonay,et al.  Measurement of greenhouse gas emissions from agricultural sites using open-path optical remote sensing method , 2009, Journal of environmental science and health. Part A, Toxic/hazardous substances & environmental engineering.