Formation of periodic disruptions induced by heat accumulation of femtosecond laser pulses.

The absorption and heat accumulation of successive ultrashort laser pulses in fused silica leads to melting of the material. We analyze the structure and formation of disruptions that occur within the trace of the molten material. We employed focused ion beam (FIB) milling to reveal the inner structure of these disruptions. The disruptions consist of several small voids which form a large cavity with a diameter of several tens of micrometer. Based on the observations, we suggest a model explaining the formation of these disruptions as a results of a fast quenching process of the molten material after the laser irradiation has stopped. In addition, we analyzed the periodic and non-periodic formation of disruptions. The processing parameters strongly influence the formation of disruptions.

[1]  A. Miotello,et al.  Contribution of vaporization and boiling to thermal-spike sputtering by ions or laser pulses. , 1999, Physical review. E, Statistical physics, plasmas, fluids, and related interdisciplinary topics.

[2]  J. Sambles,et al.  Slow waves caused by cuts perpendicular to a single subwavelength slit in metal , 2007 .

[3]  R. Waxler,et al.  Relation between refractive index and density of glasses resulting from annealing compared with corresponding relation resulting from compression. , 1966, Applied optics.

[4]  J. Nishii,et al.  Space-selective laser joining of dissimilar transparent materials using femtosecond laser pulses , 2006 .

[5]  Andreas Tünnermann,et al.  Ultra-short pulse propagation in complex optical systems. , 2005, Optics express.

[6]  A. Tünnermann,et al.  Bonding of glass with femtosecond laser pulses at high repetition rates , 2011 .

[7]  K Miura,et al.  Observation of pressure wave generated by focusing a femtosecond laser pulse inside a glass. , 2007, Optics express.

[8]  B. Poumellec,et al.  Femtosecond laser irradiation stress induced in pure silica. , 2003, Optics express.

[9]  M. Planck,et al.  Pearl-chain waveguides written at megahertz repetition rate , 2007 .

[10]  Stephen Ho,et al.  Transition from thermal diffusion to heat accumulation in high repetition rate femtosecond laser writing of buried optical waveguides. , 2008, Optics express.

[11]  F. Yoshino,et al.  Fusion Welding of Glass Using Femtosecond Laser Pulses with High-repetition Rates , 2007 .

[12]  Thomas R Huser,et al.  Modification of the fused silica glass network associated with waveguide fabrication using femtosecond laser pulses , 2003 .

[13]  Ae Williams Engineering in glass , 1951 .

[14]  E. Mazur,et al.  Bulk heating of transparent materials using a high-repetition-rate femtosecond laser , 2003 .

[15]  E. Mazur,et al.  Ultrafast-laser driven micro-explosions in transparent materials , 1997 .

[16]  M. Withford,et al.  Femtosecond laser direct-writing of waveguide Bragg gratings in a quasi cumulative heating regime. , 2011, Optics express.

[17]  Stefan Nolte,et al.  Discrete optics in femtosecond-laser-written photonic structures , 2010 .

[18]  Y. Shimotsuma,et al.  Self-organized nanogratings in glass irradiated by ultrashort light pulses. , 2003, Physical review letters.

[19]  Ya Cheng,et al.  Standing electron plasma wave mechanism of void array formation inside glass by femtosecond laser irradiation , 2007 .

[20]  Masaaki Sakakura,et al.  Mechanism of heat-modification inside a glass after irradiation with high-repetition rate femtosecond laser pulses , 2010 .

[21]  Saulius Juodkazis,et al.  Laser-matter interaction in the bulk of a transparent solid: confined microexplosion and void formation , 2006 .

[22]  J. P. Callan,et al.  Three-dimensional optical storage inside transparent materials. , 1996, Optics letters.

[23]  J. Nishii,et al.  Optical seizing and merging of voids in silica glass with infrared femtosecond laser pulses. , 2000, Optics letters.

[24]  K. Itoh,et al.  Ultrafast Processes for Bulk Modification of Transparent Materials , 2006 .

[25]  E. Mazur,et al.  Femtosecond laser micromachining in transparent materials , 2008 .

[26]  Kazuyoshi Itoh,et al.  In situ Micro-Raman Investigation of Spatio-Temporal Evolution of Heat in Ultrafast Laser Microprocessing of Glass , 2012 .

[27]  E Audouard,et al.  Single-pulse ultrafast laser imprinting of axial dot arrays in bulk glasses. , 2011, Optics letters.

[28]  R. Graf,et al.  Pearl-chain waveguides written at megahertz repetition rate , 2007 .

[29]  Yves Bellouard,et al.  Femtosecond-laser generation of self-organized bubble patterns in fused silica. , 2011, Optics express.

[30]  Saulius Juodkazis,et al.  Laser-induced microexplosion confined in a bulk of silica: formation of nanovoids , 2006 .

[31]  Andreas Tünnermann,et al.  On the fundamental structure of femtosecond laser‐induced nanogratings , 2012 .

[32]  Saulius Juodkazis,et al.  Void formation in glasses , 2007 .

[33]  Saulius Juodkazis,et al.  Time-resolved interferometry of femtosecond-laser-induced processes under tight focusing and close-to-optical breakdown inside borosilicate glass. , 2011, Optics express.