Static and transient analysis of a medium-sized sodium cooled fast reactor loaded with oxide, nitride, carbide and metallic fuels

Abstract Transient analysis was performed for the BN600 reactor loaded with different types of fuels. In order to obtain core performance parameters and major reactivity coefficients needed for transient analysis, a Serpent model based on geometrical details of the BN600 sodium-cooled fast reactor (SFR) was first created. MOX, (U-Pu) N, (U-Pu) C and (U-Pu) Fs, as representatives of oxide, nitride, carbide and metallic fuels, were loaded into this Serpent model individually. Plutonium contents were adjusted to 16.3, 14.3, 14.5 and 12.6 wt.% for these fuel cases respectively, aiming at the self-sustainability of plutonium. The safety performances of different fuel cases during the unprotected loss of flow (ULOF) and unprotected transient over power (UTOP) transients were then assessed by applying the TRACE code. The point kinetic calculation module in our TRACE model is constructed with safety related parameters obtained from our Serpent calculations. Based on our transient simulation results, comparing to other fuel cases, our nitride fuel case was proved to be able to provide the biggest margin to the working limits defined in this paper, concerning fuel melting, cladding rupture and coolant boiling. This enables the nitride fuel to be a competitive candidate for the BN600 type sodium cooled fast reactor usage.

[1]  Thermal Properties of Irradiated UO 2 and MOX , 2012 .

[2]  Christian Duriez,et al.  Thermal conductivity of hypostoichiometric low Pu content (U,Pu)O2−x mixed oxide , 2000 .

[3]  J. Noirot,et al.  HIGH BURNUP CHANGES IN UO₂ FUELS IRRADIATED UP TO 83 GWD/T IN M5 ® CLADDINGS , 2009 .

[4]  T. Fei,et al.  Neutronics Benchmark Specifications for EBR-II Shutdown Heat Removal Test SHRT-45R - Revision 1 , 2013 .

[5]  W. Dienst Swelling, densification and creep of (U, Pu)C fuel under irradiation , 1984 .

[6]  D. D. Lanning,et al.  FRAPCON-3: Modifications to fuel rod material properties and performance models for high-burnup application , 1997 .

[7]  W. M. Olson,et al.  THE DECOMPOSITION PRESSURE AND MELTING POINT OF URANIUM MONONITRIDE1 , 1963 .

[8]  J. Wallenius,et al.  Transmutation of americium in a medium size sodium cooled fast reactor design , 2010 .

[9]  T. Abe,et al.  2.15 – Uranium Oxide and MOX Production , 2012 .

[10]  P. Lam,et al.  Performance of U--Pu--Zr metal fuel in 1000 MWe LMFBRs , 1979 .

[11]  L. Leibowitz,et al.  Thermal conductivity and thermal expansion of stainless steels D9 and HT9 , 1988 .

[12]  K. Maeda,et al.  Fission gas release in FBR MOX fuel irradiated to high burnup , 2005 .

[13]  F. Oetting The chemical thermodynamic properties of nuclear materials III. Plutonium mononitride , 1972 .

[14]  Merja Pukari Experimental and theoretical studies of nitride fuels , 2013 .

[15]  D. O'Sullivan Book reviewInfluence of radiation on material properties: Proceedings of the 13th International Symposium on Effects of Radiation on Materials, held in Seattle, WA, U.S.A., June 1986 (Part 2), STP 956 , 1988 .

[16]  Pavel V. Tsvetkov,et al.  Fast spectrum reactors , 2012 .

[17]  T. Iwai,et al.  Fission gas release and swelling in uranium–plutonium mixed nitride fuels , 2004 .

[18]  J. Wallenius,et al.  Transmutation of americium in a large sized sodium-cooled fast reactor loaded with nitride fuel , 2013 .

[19]  Robert Hill,et al.  The design rationale of the IFR , 1997 .

[20]  Albert B. Reynolds,et al.  Fast breeder reactors , 1981 .

[21]  Syed E. Hasan,et al.  Thermophysical Properties Of Rocks , 1978 .

[22]  G. Hofman,et al.  Metallic Fast Reactor Fuels , 2006 .

[23]  H. S. Kamath,et al.  Fabrication, characterization and property evaluation of mixed carbide fuels for a test Fast Breeder Reactor , 2006 .

[24]  Swelling and microstructure of austenitic stainless steel ChS-68 CW after high dose neutron irradiation , 2009 .

[25]  A. I. Kiryushin,et al.  Operation experience of the BN-600 fast reactor , 1997 .

[26]  J. Fink Enthalpy and heat capacity of the actinide oxides , 1982 .

[27]  R. Konings,et al.  Comprehensive Nuclear Materials , 2012 .

[28]  W. M. Olson,et al.  The Decomposition Pressure of Plutonium Nitride1 , 1964 .

[29]  J. Philip,et al.  Irradiation Behavior of FBTR Mixed Carbide Fuel at Various Burn-ups , 2011 .

[30]  D. G. Martin,et al.  The thermal expansion of solid UO2 and (U, Pu) mixed oxides — a review and recommendations , 1988 .

[31]  R. Thetford,et al.  The chemistry and physics of modelling nitride fuels for transmutation , 2003 .

[32]  T. Matsui,et al.  Thermodynamic properties of uranium nitride, plutonium nitride and uranium-plutonium mixed nitride , 1987 .

[33]  H. Matzke,et al.  A Pragmatic Approach to Modelling Thermal Conductivity of Irradiated UO2 Fuel. Review and Recommendations , 1996 .

[34]  Mamoru Konomura,et al.  Design challenges for sodium cooled fast reactors , 2007 .