Viscoelastic flow past a confined cylinder of a low-density polyethylene melt

The capabilities of the exponential version of the Phan-Thien-Tanner (PTT) model and the Giesekus model to predict stress fields for the viscoelastic flow of a low density polyethylene melt around a confined cylinder are investigated. Computations are based on a newly developed version of the discontinuous Galerkin method. This method gives convergent results up to a Deborah number of 2.5 for the falling sphere in a tube benchmark problem. Moreover, the specific implicit-explicit implementation allows the efficient resolution of problems with multiple relaxation times which are mandatory for polymer melts. Experimentally, stress fields are related to birefringence distributions by means of the stress optical rule. Three different fits, of equal quality, to available viscometric shear data are used: two for the PTT model and one for the Giesekus model. Comparison of computed and measured fringes reveals that neither of the models is capable of describing the full birefringence pattern sufficiently well. In particular it appears difficult to predict both the birefringent tail at the wake of the cylinder that is dominated by elongational effects and the fringe pattern between cylinder and the walls where a combined shear-elongational flow is present.

[1]  Barrie Carlton Stockley,et al.  Photoelastic Stress Analysis , 1974 .

[2]  M. Mackley,et al.  The experimental observation and numerical prediction of planar entry flow and die swell for molten polyethylenes , 1995 .

[3]  R. Armstrong,et al.  Finite element analysis of steady viscoelastic flow around a sphere in a tube: calculations with constant viscosity models , 1993 .

[4]  P. P. Tas Film blowing : from polymer to product , 1994 .

[5]  F. Baaijens Numerical experiments with a discontinuous galerkin method including monotonicity enforcement on the stick-slip problem , 1994 .

[6]  Marcel Crochet,et al.  The Vortex Growth of a K.b.k.z. Fluid in An Abrupt Contraction , 1988 .

[7]  K. Walters RECENT DEVELOPMENTS IN RHEOMETRY , 1992 .

[8]  L. J. Cox Ellipsometry and Polarized Light , 1978 .

[9]  A. Isayev,et al.  Two-dimensional viscoelastic flows: experimentation and modeling , 1985 .

[10]  F. Baaijens,et al.  Application of low-order Discontinuous Galerkin methods to the analysis of viscoelastic flows , 1994 .

[11]  M.A. Hulsen,et al.  NUMERICAL SIMULATION OF CONTRACTION FLOWS USING A MULTI-MODE GIESEKUS MODEL , 1991 .

[12]  M. Fortin,et al.  A new mixed finite element method for computing viscoelastic flows , 1995 .

[13]  R. Armstrong,et al.  Finite element methdos for calculation of steady, viscoelastic flow using constitutive equations with a Newtonian viscosity , 1990 .

[14]  M. Mackley,et al.  Experimental centreline planar extension of polyethylene melt flowing into a slit die , 1995 .

[15]  E. Mitsoulis,et al.  A numerical study of the effect of elongational viscosity on vortex growth in contraction flows of polyethylene melts , 1990 .

[16]  N. Hudson,et al.  The Al project—an overview , 1993 .

[17]  J. Agassant,et al.  Steady flow of a white-metzner fluid in a 2-D abrupt contraction: computation and experiments , 1992 .

[18]  G. McKinley,et al.  The sedimentation of a sphere through an elastic fluid. Part 1. Steady motion , 1995 .

[19]  C. Han,et al.  Studies of converging flows of viscoelastic polymeric melts. II. Velocity measurements in the entrance region of a sharp‐edged slit die , 1973 .

[20]  C. Han,et al.  Studies of converging flows of viscoelastic polymeric melts. I. Stress‐birefringent measurements in the entrance region of a sharp‐edged slit die , 1973 .

[21]  F. Baaijens,et al.  Numerical analysis of start-up planar and axisymmetric contraction flows using multi-mode differential constitutive models , 1993 .

[22]  G. Fuller,et al.  Note: Optical Rheometry Using a Rotary Polarization Modulator , 1989 .

[23]  M. Fortin,et al.  A new approach for the FEM simulation of viscoelastic flows , 1989 .

[24]  Robert A. Brown,et al.  Report on the VIIIth international workshop on numerical methods in viscoelastic flows , 1994 .

[25]  C. Han,et al.  Studies of converging flows of viscoelastic polymeric melts. III. Stress and velocity distributions in the entrance region of a tapered slit die , 1973 .

[26]  F. Baaijens,et al.  An experimental and numerical investigation of a viscoelastic flow around a cylinder , 1994 .

[27]  F. Baaijens,et al.  Viscoelastic flow past a confined cylinder of a polyisobutylene solution , 1995 .

[28]  Robert C. Armstrong,et al.  A new mixed finite element method for viscoelastic flows governed by differential constitutive equations , 1995 .

[29]  O. O. O. D. Camp Identification algorithms for time-dependent materials , 1996 .

[30]  M. Crochet,et al.  A new mixed finite element for calculating viscoelastic flow , 1987 .

[31]  S. White,et al.  Numerical simulation studies of the planar entry flow of polymer melts , 1988 .

[32]  M. Mackay,et al.  Flow visualization in rheometry , 1998 .

[33]  M. Crochet,et al.  High-order finite element methods for steady viscoelastic flows , 1995 .

[34]  K. Funatsu,et al.  Numerical simulation of converging flow of polymer melts through a tapered slit die , 1993 .

[35]  E. Mitsoulis,et al.  A study of stress distribution in contraction flows of anb LLDPE melt , 1993 .