A microscopic model of electrorheology

An electrorheological fluid is modeled as a concentrated suspension of hard spheres with aligned field‐induced electric dipole moments. The presence of dipole moments causes clustering of the particles into an anisotropic suspension characterized by a particle probability distribution function. The elastic shear modulus and the dynamic viscosity are calculated from a perturbation to the particle distribution as a result of a small amplitude, high frequency, oscillatory flow. The high frequency elastic shear modulus and the dynamic viscosity are shown as a function of particle concentration and electric dipole strength. Both the modulus and the viscosity increase strongly with particle concentration. Dynamic viscosity is insensitive to dipole strength, but elastic shear modulus increases strongly with dipole strength indicating the relative importance of the particle distribution to elastic properties. The results of these calculations provide insight into the relationship between the macroscopic propertie...

[1]  D. D. Yue,et al.  Theory of Electric Polarization , 1974 .

[2]  W. Russel,et al.  Brownian Motion of Small Particles Suspended in Liquids , 1981 .

[3]  A. Hippel,et al.  Dielectrics and Waves , 1966 .

[4]  G. Batchelor The effect of Brownian motion on the bulk stress in a suspension of spherical particles , 1977, Journal of Fluid Mechanics.

[5]  Sangtae Kim,et al.  The resistance and mobility functions of two equal spheres in low‐Reynolds‐number flow , 1985 .

[6]  S. G. Mason,et al.  Some electrohydrodynamic effects in fluid dispersions , 1980 .

[7]  W. Russel Review of the Role of Colloidal Forces in the Rheology of Suspensions , 1980 .

[8]  G. Batchelor,et al.  Brownian diffusion of particles with hydrodynamic interaction , 1976, Journal of Fluid Mechanics.

[9]  G. V. Vinogradov,et al.  Electric fields in the rheology of disperse systems , 1984 .

[10]  J. Hayter,et al.  A comparison of molecular dynamics and analytic calculation of correlations in an aligned ferrofluid , 1984 .

[11]  D. Jeffrey,et al.  Conduction through a random suspension of spheres , 1973, Proceedings of the Royal Society of London. A. Mathematical and Physical Sciences.

[12]  J. Hayter,et al.  Structure Factor of a Magnetically Saturated Ferrofluid , 1982 .

[13]  John F. Brady,et al.  Dynamic simulation of sheared suspensions. I. General method , 1984 .

[14]  P. Mazur,et al.  Diffusion of spheres in a concentrated suspension : resummation of many-body hydrodynamic interactions , 1983 .

[15]  J. Turner,et al.  Two-phase conductivity: The electrical conductance of liquid-fluidized beds of spheres , 1976 .

[16]  A. Gast,et al.  Nonequilibrium statistical mechanics of concentrated colloidal dispersions: Hard spheres in weak flows , 1986 .

[17]  B. J. Yoon,et al.  Note on the direct calculation of mobility functions for two equal-sized spheres in Stokes flow , 1987, Journal of Fluid Mechanics.

[18]  W. M. Winslow Induced Fibration of Suspensions , 1949 .