Influences of the 2010 Eyjafjallajökull volcanic plume on air quality in the northern Alpine region

Abstract. A series of major eruptions of the Eyjafjallajokull volcano in Iceland started on 14 April 2010 and continued until the end of May 2010. The volcanic emissions moved over nearly the whole of Europe and were observed first on 16 April 2010 in Southern Germany with different remote sensing systems from the ground and space. Enhanced PM10 and SO2 concentrations were detected on 17 April at mountain stations (Zugspitze/Schneefernerhaus and Schauinsland) as well as in Innsbruck by in situ measurement devices. On 19 April intensive vertical mixing and advection along with clear-sky conditions facilitated the entrainment of volcanic material down to the ground. The subsequent formation of a stably stratified lower atmosphere with limited mixing near the ground during the evening of 19 April led to an additional enhancement of near-surface particle concentrations. Consequently, on 19 April and 20 April exceedances of the daily threshold value for particulate matter (PM10) were reported at nearly all monitoring stations of the North Alpine foothills as well as at mountain and valley stations in the northern Alps. The chemical analyses of ambient PM10 at monitoring stations of the North Alpine foothills yielded elevated Titanium concentrations on 19/20 April which prove the presence of volcanic plume material. Following this result the PM10 threshold exceedances are also associated with the volcanic plume. The entrainment of the volcanic plume material mainly affected the concentrations of coarse particles (>1 μm) – interpreted as volcanic ash – and ultrafine particles (

[1]  J. Kerkmann,et al.  Simultaneous retrieval of volcanic ash and SO2 using MSG-SEVIRI measurements , 2007 .

[2]  B. Brunekreef,et al.  Air pollution and health , 2002, The Lancet.

[3]  A. Kibble,et al.  Syndromic surveillance to assess the potential public health impact of the Icelandic volcanic ash plume across the United Kingdom, April 2010. , 2010, Euro surveillance : bulletin Europeen sur les maladies transmissibles = European communicable disease bulletin.

[4]  P. Rossini,et al.  April-May 2010 Eyjafjallajökull volcanic fallout over Rimini, Italy , 2012 .

[5]  K. Lehtinen,et al.  Changes in the production rate of secondary aerosol particles in Central Europe in view of decreasing SO 2 emissions between 1996 and 2006 , 2009 .

[6]  A. Peters,et al.  Particle size distribution factor as an indicator for the impact of the Eyjafjallajökull ash plume at ground level in Augsburg, Germany , 2011 .

[7]  H. Wichmann,et al.  COMPARISON OF THE NUMBER OF ULTRA-FINE PARTICLES AND THE MASS OF FINE PARTICLES WITH RESPIRATORY SYMPTOMS IN ASTHMATICS , 1997 .

[8]  Guðrún Nína Petersen,et al.  A short meteorological overview of the Eyjafjallajökull eruption 14 April–23 May 2010 , 2010 .

[9]  Douglas W Dockery,et al.  Health effects of particulate air pollution. , 2009, Annals of epidemiology.

[10]  Stefan Emeis,et al.  Remote Sensing Methods to Investigate Boundary-layer Structures relevant to Air Pollution in Cities , 2006 .

[11]  Hanna Vehkamäki,et al.  Formation and growth rates of ultrafine atmospheric particles: a review of observations , 2004 .

[12]  Chunsheng Zhao,et al.  Mobility particle size spectrometers: harmonization of technical standards and data structure to facilitate high quality long-term observations of atmospheric particle number size distributions , 2010 .

[13]  Stephen Self,et al.  Atmospheric and environmental effects of the 1783-1784 Laki eruption: A review and reassessment , 2003 .

[14]  U. Schumann,et al.  Airborne observations of the Eyjafjalla volcano ash cloud over Europe during air space closure in April and May 2010 , 2010 .

[15]  E. Naumova,et al.  Emergency room visits for respiratory conditions in children increased after Guagua Pichincha volcanic eruptions in April 2000 in Quito, Ecuador Observational Study: Time Series Analysis , 2007, Environmental health : a global access science source.

[16]  V. Dietze,et al.  Geochemical characterization of single atmospheric particles from the Eyjafjallajökull volcano eruption event collected at ground-based sampling sites in Germany , 2012 .

[17]  Alfred J Prata,et al.  Observations of volcanic ash clouds in the 10-12 μm window using AVHRR/2 data , 1989 .

[18]  A. Peters,et al.  Particulate Matter Air Pollution and Cardiovascular Disease: An Update to the Scientific Statement From the American Heart Association , 2010, Circulation.

[19]  M. Haeffelin,et al.  Assessing in near real time the impact of the April 2010 Eyjafjallajökull ash plume on air quality , 2011 .

[20]  A. Stohl,et al.  Volcanic aerosol optical properties and phase partitioning behavior after long-range advection characterized by UV-Lidar measurements , 2012 .

[21]  A. Stohl,et al.  Determination of time-and height-resolved volcanic ash emissions for quantitative ash dispersion modeling : the 2010 Eyjafjallajökull eruption , 2011 .

[22]  Josef Gasteiger,et al.  Volcanic ash from Iceland over Munich: mass concentration retrieved from ground-based remote sensing measurements , 2010 .

[23]  Albert Ansmann,et al.  Simulations of the 2010 Eyjafjallajökull volcanic ash dispersal over Europe using COSMO–MUSCAT , 2012 .

[24]  W. Birmili,et al.  The Hohenpeissenberg aerosol formation experiment (HAFEX): a long-term study including size-resolved aerosol, H 2 SO 4 , OH, and monoterpenes measurements , 2002 .

[25]  J. Schwartz,et al.  The Effect of Fine and Coarse Particulate Air Pollution on Mortality: A National Analysis , 2009, Environmental health perspectives.

[26]  U. Lohmann,et al.  Aerosol nucleation and its role for clouds and Earth's radiative forcing in the aerosol-climate model ECHAM5-HAM , 2010 .

[27]  T. Thordarson,et al.  The Laki (Skaftár Fires) and Grímsvötn eruptions in 1783–1785 , 1993 .

[28]  E. Zaady,et al.  Dust storm originate from Sahara covering Western Europe: A case study , 2008 .

[29]  Makiko Sato,et al.  Potential climate impact of Mount Pinatubo eruption , 1992 .

[30]  M. Brayshay,et al.  An Amazing and Portentous Summer: Environmental and Social Responses in Britain to the 1783 Eruption of an Iceland Volcano , 1995 .

[31]  C. Oppenheimer,et al.  Near-source observations of aerosol size distributions in the eruptive plumes from Eyjafjallajökull volcano, March–April 2010 , 2011 .

[32]  T. Ishizuka,et al.  Acute Impact of Volcanic Ash on Asthma Symptoms and Treatment , 2007, International journal of immunopathology and pharmacology.

[33]  Wei Yang,et al.  Acute Health Effects Associated with Exposure to Volcanic Air Pollution (vog) from Increased Activity at Kilauea Volcano in 2008 , 2010, Journal of toxicology and environmental health. Part A.

[34]  A. Hansell,et al.  Health Hazards from Volcanic Gases: A Systematic Literature Review , 2004, Archives of environmental health.

[35]  John R. Christy,et al.  THE IMPACT OF MOUNT PINATUBO ON WORLD‐WIDE TEMPERATURES , 1996 .

[36]  Ralf Zimmermann,et al.  Seasonal and diurnal variation of PM2.5 apparent particle density in urban air in Augsburg, Germany. , 2008, Environmental science & technology.

[37]  Annette Peters,et al.  Spatial and temporal variation of particle number concentration in Augsburg, Germany. , 2008, The Science of the total environment.

[38]  G. Gudmundsson Respiratory health effects of volcanic ash with special reference to Iceland. A review , 2011, The clinical respiratory journal.

[39]  W. Junkermann,et al.  An Ultralight Aircraft as Platform for Research in the Lower Troposphere: System Performance and First Results from Radiation Transfer Studies in Stratiform Aerosol Layers and Broken Cloud Conditions , 2001 .

[40]  Stefan Emeis,et al.  Measurement and simulation of the 16/17 April 2010 Eyjafjallajökull volcanic ash layer dispersion in the northern Alpine region , 2011 .

[41]  M. Facchini,et al.  On the roles of sulphuric acid and low-volatility organic vapours in the initial steps of atmospheric new particle formation , 2010 .

[42]  B. Brunekreef,et al.  Epidemiological evidence of effects of coarse airborne particles on health , 2005, European Respiratory Journal.

[43]  Rebecca Bascom,et al.  Health effects of outdoor air pollution , 1996 .

[44]  M. Pujadas,et al.  Characterization of the Eyjafjallajökull volcanic plume over the Iberian Peninsula by lidar remote sensing and ground-level data collection , 2012 .

[45]  M. Macchiato,et al.  Eyjafjallajökull volcanic ash in southern Italy , 2012 .

[46]  Michal Krzyzanowski,et al.  Air Pollution and Public Health: A Guidance Document for Risk Managers , 2008, Journal of toxicology and environmental health. Part A.

[47]  H. Tong,et al.  Differential Cardiopulmonary Effects of Size-Fractionated Ambient Particulate Matter in Mice , 2010, Cardiovascular Toxicology.

[48]  C. O'Dowd,et al.  Particle mobility size spectrometers : harmonization of technical standards and data structure to facilitate high quality long-term observations of atmospheric particle number size distributions , 2010 .

[49]  Kerstin Stebel,et al.  Determination of time- and height-resolved volcanic ash emissions and their use for quantitative ash dispersion modeling: the 2010 Eyjafjallajökull eruption , 2011 .

[50]  Arnau Folch,et al.  Volcanic ash over Europe during the eruption of Eyjafjallajökull on Iceland, April–May 2010 , 2012 .

[51]  A. J. Prata,et al.  Sulphur dioxide as a volcanic ash proxy during the April–May 2010 eruption of Eyjafjallajökull Volcano, Iceland , 2011 .

[52]  V. Freudenthaler,et al.  Spatial structure and dispersion of the 16/17 April 2010 volcanic ash cloud over Germany. , 2010 .

[53]  A. Peters,et al.  Quality control and quality assurance for particle size distribution measurements at an urban monitoring station in Augsburg, Germany. , 2008, Journal of environmental monitoring : JEM.

[54]  S. Gilge,et al.  Assessment of the applicability of NO-NO 2 -O 3 photostationary state to long-term measurements at the Hohenpeissenberg GAW Station, Germany , 2004 .

[55]  J. Schmetz,et al.  AN INTRODUCTION TO METEOSAT SECOND GENERATION (MSG) , 2002 .

[56]  W. Steinbrecht,et al.  The Eyjafjallajökull eruption in April 2010 – detection of volcanic plume using in-situ measurements, ozone sondes and lidar-ceilometer profiles , 2010 .