Local heat generated by a focused He+ ion beam

A focused He+ beam with a beam diameter less than 1 nm is heating up the targeted surface for a He+ dose larger than 1 × 1020 ions cm−2. The temperature can reach 1000 °C locally, resulting in surface decomposition or chemical reactions. This temperature was measured by fabricating gold nanodisks down to 20 nm in diameter and 10 nm in thickness on mica and sapphire surfaces. The melting and vaporization of these nanodisks were used to determine this temperature according to the known gold nanocluster melting temperature variations as a function of their volume. This local heat production is very negative for precise He+ nanolithography resist processes but advantageous without a resist when used to directly nano-sculpture a nanomaterial when a very thermally conductive support like sapphire is selected.

[1]  D. Mailly,et al.  Three-Dimensional Superconducting Nanohelices Grown by He+-Focused-Ion-Beam Direct Writing , 2019, Nano letters.

[2]  M. Aono,et al.  Observation of room temperature electronic localization through a single graphene layer on sapphire , 2019, Japanese Journal of Applied Physics.

[3]  P. Rack,et al.  Review Article: Advanced nanoscale patterning and material synthesis with gas field helium and neon ion beams , 2017 .

[4]  T. Iijima,et al.  Direct nano-patterning of graphene with helium ion beams , 2015 .

[5]  N. Yokoyama,et al.  Conduction tuning of graphene based on defect-induced localization. , 2013, ACS nano.

[6]  A. Mahmood,et al.  Side-gated transport in focused-ion-beam-fabricated multilayered graphene nanoribbons. , 2007, Small.

[7]  Amit Misra,et al.  Influence of interfaces on the storage of ion-implanted He in multilayered metallic composites , 2005 .

[8]  G. Schmid,et al.  Nanoparticulated Gold: Syntheses, Structures, Electronics, and Reactivities , 2003 .

[9]  Yoshio Bando,et al.  Carbon nanothermometer containing gallium , 2002, Nature.

[10]  Lai,et al.  Size-Dependent Melting Properties of Small Tin Particles: Nanocalorimetric Measurements. , 1996, Physical review letters.

[11]  P. Buffat,et al.  Size effect on the melting temperature of gold particles , 1976 .

[12]  Mieko Takagi,et al.  Electron-Diffraction Study of Liquid-Solid Transition of Thin Metal Films , 1954 .

[13]  O. Vyvenko,et al.  Secondary Electron Generation in the Helium Ion Microscope: Basics and Imaging , 2016 .

[14]  R. A. Bayles,et al.  Small particle melting of pure metals , 1986 .