Lead–lithium eutectic material database for nuclear fusion technology

Abstract Fully validated material databases are needed for coherent technological developments in any R&D field. For nuclear fusion technology (NFT), within a near-term perspective of qualification and licensing of nuclear components and systems, this goal is both compulsory and urgent. This mandatory requirement applies for the particular case of the Pb–Li eutectic database as fusion reactor material. Pb16Li is today a reference breeder material in diverse fusion R&D programs worldwide. Technical consensus on most part of the material database inputs seems a major technological objective. In this work Pb16Li material database inputs for NFT have been systematically reviewed. Database inputs (bulk, thermal, physical-chemistry properties, and H-isotopes transport) are discussed and extended to base magnetohydrodynamic (MHD) properties, values for non-dimensional parameters and pipe/channel correlations in 2-phases dispersion models. Ongoing efforts to develop the Pb16Li material database as a computing expert system are reported.

[1]  P. Fauvet,et al.  Hydrogen behaviour in liquid 17Li83Pb alloy , 1988 .

[2]  T. Sample,et al.  Thermodynamics of Pb17Li-bismuth interactions , 1994 .

[3]  F. Reiter,et al.  Solubility and diffusivity of hydrogen isotopes in liquid Pb17Li , 1991 .

[4]  S. Lai,et al.  Theoretical study of the temperature dependences of electronic magnetic susceptibilities for liquid lithium and sodium , 1991 .

[5]  F. Yoshida Bubble column research in Japan , 1988 .

[6]  Y. Fujii,et al.  Isothermal release of tritium from neutron-irradiated Li17Pb83 , 1987 .

[7]  S. Stankus,et al.  An experimental investigation of the density and thermal expansion of advanced materials and heat-transfer agents of liquid-metal systems of fusion reactor: Lead-lithium eutectic , 2006 .

[8]  T. Sample,et al.  The solubilities of nickel, manganese and chromium in Pb17Li , 1991 .

[9]  Martensitic transformation of lithium: Magnetic susceptibility measurements , 1997 .

[10]  H. Feuerstein,et al.  Self-adjustment of Li in Pb-17Li systems , 1998 .

[11]  H. Katsuta,et al.  Hydrogen solubility in liquid Li17Pb83 , 1985 .

[12]  E. Seymour,et al.  Magnetic properties of lead alloys in the solid and liquid states (NMR) , 1972 .

[13]  Andrea Ciampichetti,et al.  Determination of hydrogen solubility in lead lithium using sole device , 2006 .

[14]  P. Hubberstey Pb17Li and lithium: A thermodynamic rationalisation of their radically different chemistry , 1997 .

[15]  C. Wu The solubility of deuterium in lithium-lead alloys , 1983 .

[16]  T. Terai,et al.  Modeling of In-Pile Experiments on Tritium Release from Molten Lithium-Lead , 2002 .

[17]  T. Sample,et al.  Thermodynamics of Pb-17Li-bismuth interactions , 1994 .

[18]  T. Terai,et al.  Diffusion coefficient of tritium in molten lithium-lead alloy (Li17Pb83) under neutron irradiation at elevated temperatures , 1992 .

[19]  Robert E. Buxbaum,et al.  A chemical theory analysis of the solution thermodynamics of oxygen, nitrogen and hydrogen in lead-rich LiPb mixtures , 1984 .

[20]  E. Veleckis,et al.  A thermodynamic investigation of dilute solutions of hydrogen in liquid Li-Pb alloys , 1984 .

[21]  S. Zinkle,et al.  Thermodynamic stability of oxide, nitride, and carbide coating materials in liquid Sn-25Li , 2004 .

[22]  B. Schulz,et al.  Thermophysical properties of the Li(17)Pb(83)alloy , 1991 .

[23]  Anton Möslang,et al.  Development of self-cooled liquid metal breeder blankets , 1995 .