Measurements of Saharan dust aerosols over the Eastern Mediterranean using elastic backscatter-Raman lidar, spectrophotometric and satellite observations in the frame of the EARLINET project

We report on the vertical distributions of Saharan dust aerosols over the N.E. Mediterranean region, which were obtained during a typical dust outbreak on August 2000, by two lidar systems located in Athens and Thessaloniki, Greece, in the frame of the European EARLINET project. MODIS and ground sun spectrophotometric data, as well as air-mass backward trajectories confirmed the existence of Saharan dust in the case examined, which was also successfully forecasted by the DREAM dust model. The lidar data analysis for the period 2000-2002 made possible, for the first time, an estimation of the vertical extent of free tropospheric dust layers [mean values of the aerosol backscatter and extinction coefficients and the extinction-to-backscatter ratio (lidar ratio, LR) at 355 nm], as well as a seasonal distribution of Saharan dust outbreaks over Greece, under cloud-free conditions. A mean value of the lidar ratio at 355 nm was obtained over Athens (53±1 sr) and over Thessaloniki (44±2 sr) during the Saharan dust outbreaks. The corresponding aerosol optical thickness (AOT) at 355 nm, in the altitude range 0-5 km, was 0.69±0.12 and 0.65±0.10 for Athens and Thessaloniki, respectively (within the dust layer the AOT was 0.23 and 0.21, respectively). Air-mass back-trajectory analysis performed in the period 2000-2002 for all Saharan dust outbreaks over the N.E. Mediterranean indicated the main pathways followed by the dust aerosols.

[1]  J. Ackermann The Extinction-to-Backscatter Ratio of Tropospheric Aerosol: A Numerical Study , 1998 .

[2]  M. Mishchenko,et al.  Modeling phase functions for dustlike tropospheric aerosols using a shape mixture of randomly oriented polydisperse spheroids , 1997 .

[3]  J. P. Díaz,et al.  Radiative transfer modeling in the UV-VIS region with the presence of Saharan mineral desert aerosols , 2000 .

[4]  D. Roy,et al.  Achieving sub-pixel geolocation accuracy in support of MODIS land science , 2002 .

[5]  Takashi Shibata,et al.  Case study of Raman lidar measurements of Asian dust events in 2000 and 2001 at Nagoya and Tsukuba, Japan , 2002 .

[6]  T. Eck,et al.  An emerging ground-based aerosol climatology: Aerosol optical depth from AERONET , 2001 .

[7]  Jay R. Herman,et al.  Observed effects of particles nonsphericity on the retrieval of marine and desert dust aerosol optical depth by lidar , 2002 .

[8]  A. Stohl A 1-year Lagrangian ``climatology'' of airstreams in the Northern Hemisphere troposphere and lowermost stratosphere , 2001 .

[9]  C. Hueglin,et al.  Saharan dust events at the Jungfraujoch: detection by wavelength dependence of the single scattering albedo and first climatology analysis , 2004 .

[10]  D. Tanré,et al.  Remote Sensing of Tropospheric Aerosols from Space: Past, Present, and Future. , 1999 .

[11]  G. Gobbi,et al.  Aerosol seasonal variability over the Mediterranean region and relative impact of maritime, continental and Saharan dust particles over the basin from MODIS data in the year 2001 , 2004 .

[12]  Larry L. Stowe,et al.  Characterization of tropospheric aerosols over the oceans with the NOAA advanced very high resolution radiometer optical thickness operational product , 1997 .

[13]  R. Evans,et al.  Atmospheric correction of ocean color imagery through thick layers of Saharan dust , 2001 .

[14]  Reto Knutti,et al.  Climate Forcing by Aerosols--a Hazy Picture , 2003, Science.

[15]  O. Torres,et al.  Biomass burning smoke measured using backscattered ultraviolet radiation: SCAR‐B and Brazilian smoke interannual variability , 1998 .

[16]  Y. Kaufman,et al.  Passive remote sensing of tropospheric aerosol and atmospheric , 1997 .

[17]  Philip B. Russell,et al.  ACE-ASIA Regional Climatic and Atmospheric Chemical Effects of Asian Dust and Pollution , 2004 .

[18]  C. Kottmeier,et al.  Trajectories in the Antarctic lower troposphere , 1998 .

[19]  P. Bhartia,et al.  Impact of tropospheric aerosol absorption on ozone retrieval from backscattered ultraviolet measurements , 1999 .

[20]  F. Dulac,et al.  Airborne study of a multi-layer aerosol structure in the eastern Mediterranean observed with the airborne polarized lidar ALEX during a STAAARTE campaign (7 June 1997) , 2003 .

[21]  Mian Chin,et al.  Long-term simulation of global dust distribution with the GOCART model: correlation with North Atlantic Oscillation , 2004, Environ. Model. Softw..

[22]  J. Seinfeld,et al.  Atmospheric Chemistry and Physics: From Air Pollution to Climate Change , 1997 .

[23]  Toby N. Carlson,et al.  Saharan air outbreaks over the tropical North Atlantic , 1980 .

[24]  A. Ansmann,et al.  Aerosol lidar intercomparison in the framework of the EARLINET project. 3. Raman lidar algorithm for aerosol extinction, backscatter, and lidar ratio. , 2004, Applied optics.

[25]  L. Mona,et al.  One year of tropospheri clidar measurements of aerosol extinction and backscatter , 2003 .

[26]  Christos Zerefos,et al.  Tropospheric LIDAR aerosol measurements and sun photometric observations at Thessaloniki, Greece , 2000 .

[27]  François Dulac,et al.  Control of atmospheric export of dust from North Africa by the North Atlantic Oscillation , 1997, Nature.

[28]  B. Holben,et al.  Aerosol load characterization over South–East Italy for one year of AERONET sun-photometer measurements , 2005 .

[29]  Albert Ansmann,et al.  Vertical profiling of optical and physical particle properties over the tropical Indian Ocean with six‐wavelength lidar: 2. Case studies , 2001 .

[30]  G. Gobbi,et al.  Altitude-resolved properties of a Saharan dust event over the Mediterranean , 2000 .

[31]  A. Ansmann,et al.  Dual‐wavelength Raman lidar observations of the extinction‐to‐backscatter ratio of Saharan dust , 2002 .

[32]  P. Crutzen,et al.  Atmospheric aerosols: Biogeochemical sources and role in atmospheric chemistry , 1997 .

[33]  M. Noguer,et al.  Climate change 2001: The scientific basis. Contribution of Working Group I to the Third Assessment Report of the Intergovernmental Panel on Climate Change , 2002 .

[34]  O. Krüger,et al.  The indirect aerosol effect over Europe , 2002 .

[35]  Albert Ansmann,et al.  Multiyear aerosol observations with dual‐wavelength Raman lidar in the framework of EARLINET , 2004 .

[36]  Alexander Ignatov,et al.  Sensitivity study of the Ångström exponent derived from AVHRR over the oceans , 1998 .

[37]  V. Freudenthaler,et al.  Long-range transport of Saharan dust to northern Europe : The 11-16 October 2001 outbreak observed with EARLINET , 2003 .

[38]  C. Moulin,et al.  Evidence of the control of summer atmospheric transport of African dust over the Atlantic by Sahel sources from TOMS satellites (1979–2000) , 2004 .

[39]  Alexander Ignatov,et al.  Development, validation, and potential enhancements to the second‐generation operational aerosol product at the National Environmental Satellite, Data, and Information Service of the National Oceanic and Atmospheric Administration , 1997 .

[40]  S. H. Melfi,et al.  Validation of the Saharan dust plume conceptual model using lidar, meteosat, and ECMWF Data , 1999 .

[41]  M. Perrone,et al.  Raman lidar monitoring of extinction and backscattering of African dust layers and dust characterization. , 2003, Applied optics.

[42]  O. Torres,et al.  ENVIRONMENTAL CHARACTERIZATION OF GLOBAL SOURCES OF ATMOSPHERIC SOIL DUST IDENTIFIED WITH THE NIMBUS 7 TOTAL OZONE MAPPING SPECTROMETER (TOMS) ABSORBING AEROSOL PRODUCT , 2002 .

[43]  G. d’Almeida,et al.  A model for Saharan dust transport , 1986 .

[44]  V. Masson,et al.  Satellite climatology of African dust transport in the Mediterranean atmosphere , 1998 .

[45]  Paolo Bonasoni,et al.  Aerosol-ozone correlations during dust transport episodes , 2004 .

[46]  M. Schrope Trouble in the greenhouse , 2000, Nature.

[47]  K. Moorthy,et al.  Radiative effects of natural aerosols: A review , 2005 .

[48]  C. Moulin,et al.  Aerosol sources and their contribution to the chemical composition of aerosols in the Eastern Mediterranean Sea during summertime , 2002 .

[49]  J. Coakley,et al.  Climate Forcing by Anthropogenic Aerosols , 1992, Science.

[50]  Albert Ansmann,et al.  Physical properties of the Indian aerosol plume derived from six‐wavelength lidar Observations on 25 March 1999 of the Indian Ocean Experiment , 2000 .

[51]  G. Stenchikov,et al.  The impact of aerosols on solar ultraviolet radiation and photochemical smog. , 1997, Science.

[52]  James N. Galloway,et al.  Atmospheric deposition of nutrients to the North Atlantic Basin. , 1996 .

[53]  A. da Silva,et al.  Quantification of dust-forced heating of the lower troposphere , 1998, Nature.

[54]  Anthony S. Wexler,et al.  Dynamics of Tropospheric Aerosols , 1995 .

[55]  P. Bhartia,et al.  Detection of biomass burning smoke from TOMS measurements , 1996 .

[56]  G. Fiocco,et al.  Saharan dust profiles measured by lidar at Lampedusa , 2001 .

[57]  Alexandros Papayannis,et al.  The EOLE Project: A multiwavelength laser remote sensing (lidar) system for ozone and aerosol measurements in the troposphere and the lower stratosphere. Part II: Aerosol measurements over Athens, Greece , 2002 .

[58]  J. Prospero Long‐term measurements of the transport of African mineral dust to the southeastern United States: Implications for regional air quality , 1999 .

[59]  Giorgio Fiocco,et al.  Direct radiative forcing of Saharan dust in the Mediterranean from measurements at Lampedusa Island and MISR space-borne observations , 2004 .

[60]  T. Eck,et al.  Wavelength dependence of the optical depth of biomass burning, urban, and desert dust aerosols , 1999 .

[61]  D. Tanré,et al.  ALGORITHM FOR REMOTE SENSING OF TROPOSPHERIC AEROSOL FROM MODIS , 1998 .

[62]  J. Lelieveld,et al.  Global Air Pollution Crossroads over the Mediterranean , 2002, Science.

[63]  Didier Tanré,et al.  Satellite Climatology of Saharan Dust Outbreaks: Method and Preliminary Results , 1992 .

[64]  G. Kallos,et al.  A model for prediction of desert dust cycle in the atmosphere , 2001 .

[65]  Remo Guidieri Res , 1995, RES: Anthropology and Aesthetics.

[66]  G. Kallos,et al.  Saharan dust contributions to PM10 and TSP levels in Southern and Eastern Spain , 2001 .

[67]  A. Ansmann,et al.  Independent measurement of extinction and backscatter profiles in cirrus clouds by using a combined Raman elastic-backscatter lidar. , 1992, Applied optics.

[68]  Heini Wernli,et al.  A 15-Year Climatology of Warm Conveyor Belts , 2004 .

[69]  A. Stohl Computation, accuracy and applications of trajectories—A review and bibliography , 1998 .

[70]  V. Salomonson,et al.  MODIS: advanced facility instrument for studies of the Earth as a system , 1989 .

[71]  Steven A. Ackerman,et al.  Radiative Effects of Airborne Dust on Regional Energy Budgets at the Top of the Atmosphere , 1992 .

[72]  D. Tanré,et al.  Assessment of the African airborne dust mass over the western Mediterranean Sea using Meteosat data , 1992 .

[73]  Alexandros Papayannis,et al.  Characterization of the vertical structure of Saharan dust export to the Mediterranean basin , 1999 .

[74]  A. Ansmann,et al.  Aerosol lidar intercomparison in the framework of the EARLINET project. 2. Aerosol backscatter algorithms. , 2004, Applied optics.

[75]  J. Klett Lidar inversion with variable backscatter/extinction ratios. , 1985, Applied optics.

[76]  C. Zerefos,et al.  Optical properties of Saharan dust layers as detected by a Raman lidar at Thessaloniki, Greece , 2004 .

[77]  C. Velden,et al.  ARTICLES: The Impact of the Saharan Air Layer on Atlantic Tropical Cyclone Activity. , 2004 .

[78]  J. Herman,et al.  Tropical tropospheric ozone and biomass burning. , 2001, Science.

[79]  Paul Ginoux,et al.  A Long-Term Record of Aerosol Optical Depth from TOMS Observations and Comparison to AERONET Measurements , 2002 .

[80]  Ulrike Lohmann,et al.  Can the direct and semi‐direct aerosol effect compete with the indirect effect on a global scale? , 2001 .

[81]  V. Freudenthaler,et al.  Aerosol lidar intercomparison in the framework of the EARLINET project. 1. Instruments. , 2004, Applied optics.

[82]  A. Ansmann,et al.  Comparison of the radiative impact of aerosols derived from vertically resolved (lidar) and vertically integrated (Sun photometer) measurements: Example of an Indian aerosol plume , 2001 .

[83]  I. Jankowiak,et al.  Long‐term daily monitoring of Saharan dust load over ocean using Meteosat ISCCP‐B2 data: 2. Accuracy of the method and validation using Sun photometer measurements , 1997 .

[84]  Eric P. Shettle,et al.  Atmospheric Aerosols: Global Climatology and Radiative Characteristics , 1991 .