This thesis consists of two parts. The main part is concerned with new schemes for measurementbased quantum computation. Computers utilizing the laws of quantum me chanics promise an exponential speed-up over purely classical devi ces. Recently, considerable attention has been paid to the measurement-ba sed p radigm of quantum computers. It has been realized that local measur ments on certain highly entangled quantum states are computational ly as powerful as the well-established model for quantum computation based o n controlled unitary evolution. Prior to this thesis, only one family of quantum states was kn own to possess this computational power: the so-called cluster state and s ome very close relatives. Questions posed and answered in this thesis incl ude: Can one find families of states different from the cluster, which con stitute universal resources for measurement-based computation? Can the high ly s ngular properties of the cluster state be relaxed while retaining u iversality? Is the quality of being a computational resource common or rare among pure states? We start by establishing a new mathematical tool for underst anding the connection between local measurements on an entangled quantum state and a quantum computation. This framework – based on finitely corr elated states (or matrix product states) common in many-body physics – is t he first such tool general enough to apply to a wide range of quantum states beyond the family of graph states. We employ it to construct a variety of new universal resource states and schemes for measurement-based c omputation. It is found that many entanglement properties of universal sta te may be radically different from those of the cluster: we identify state s which are locally arbitrarily close to a pure state, exhibit long-ranged corr elations or cannot be converted into cluster states by means of stochastic loca l operations and classical communication. Flexible schemes for the compens ation of the inherent randomness of quantum measurements are introduce d. W proceed to provide a complete classification of a natural class o f tates which can take the role of a single logical qubit in a measurement-b ased quantum computer. Lastly, it is demonstrated that states can be too e ntangled to be useful for any computational purpose. Concentration of mea sure arguments show that this problem occurs for the dramatic majority of al l pure states. The second part of the thesis is concerned with discrete quan tum phase spaces. We prove that the only pure states to possess a non-ne gative Wigner function are stabilizer states. The result can be seen as a fin ite-dimensional analogue of a classic theorem due to Hudson, who showed that G aussian states play the same role in the setting of continuous variab le systems. The quantum phase space techniques developed for this argument are subsequently used to quantize a well-known structure from classi cal computer science: the Margulis expander.
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