Life Cycle Assessment of repurposed electric vehicle batteries: an adapted method based on modelling energy flows

Abstract After their first use in electric vehicles (EVs), the residual capacity of traction batteries can make them valuable in other applications. Although reusing EV batteries remains an undeveloped market, second-use applications of EV batteries are in line with circular economy principles and the waste management hierarchy. Although substantial environmental benefits are expected from reusing traction batteries, further efforts are needed in data collection, modelling the life-cycle stages and calculating impact indicators to propose a harmonized and adapted life-cycle assessment (LCA) method. To properly assess the environmental benefits and drawbacks of using repurposed EV batteries in second-use applications, in this article an adapted LCA is proposed based on the comparison of different scenarios from a life-cycle perspective. The key issues for the selected life-cycle stages and the aspects and parameters to be assessed in the analysis are identified and discussed for each stage, including manufacturing, repurposing, reusing and recycling. The proposed method is applied to a specific case study concerning the use of repurposed batteries to increase photovoltaic (PV) self-consumption in a given dwelling. Primary data on the dwelling’s energy requirements and PV production were used to properly assess the energy flows in this specific repurposed scenario: both the literature search performed and the results obtained highlighted the relevance of modelling the system energy using real data, combining the characteristics of both the battery and its application. The LCA results confirmed that the environmental benefits of adopting repurposed batteries to increase PV self-consumption in a house occur under specific conditions and that the benefits are more or less considerable depending on the impact category assessed. Higher environmental benefits refer to impact categories dominated by the manufacturing and repurposing stages. Some of the most relevant parameters (e.g. residual capacity and allocation factor) were tested in a sensitivity analysis. The method can be used in other repurposing application cases if parameters for these cases can be determined by experimental tests, modelling or extracting data from the literature.

[1]  V. Bermudez Electricity storage supporting PV competitiveness in a reliable and sustainable electric network , 2017 .

[2]  E. Martinez-Laserna,et al.  Second life battery energy storage system for enhancing renewable energy grid integration , 2015, 2015 IEEE Energy Conversion Congress and Exposition (ECCE).

[3]  Gillian Lacey,et al.  The use of second life electric vehicle batteries for grid support , 2013, Eurocon 2013.

[4]  Erwan Saouter,et al.  Comparing chemical environmental scores using USEtox™ and CDV from the European Ecolabel , 2011 .

[5]  Amaia Iturrondobeitia,et al.  Second life of electric vehicle batteries: relation between materials degradation and environmental impact , 2015, The International Journal of Life Cycle Assessment.

[6]  B. Swain Recovery and recycling of lithium: A review , 2017 .

[7]  Lars Ole Valøen,et al.  Life Cycle Assessment of a Lithium‐Ion Battery Vehicle Pack , 2014 .

[8]  G. G. Stokes "J." , 1890, The New Yale Book of Quotations.

[9]  Andrew Burke,et al.  Performance, Charging, and Second-use Considerations for Lithium Batteries for Plug-in Electric Vehicles , 2009 .

[10]  Vilayanur V. Viswanathan,et al.  Second Use of Transportation Batteries: Maximizing the Value of Batteries for Transportation and Grid Services , 2011, IEEE Transactions on Vehicular Technology.

[11]  Hans-Jürgen Dr. Klüppel,et al.  The Revision of ISO Standards 14040-3 - ISO 14040: Environmental management – Life cycle assessment – Principles and framework - ISO 14044: Environmental management – Life cycle assessment – Requirements and guidelines , 2005 .

[12]  Michael Q. Wang,et al.  Material and energy flows in the materials production, assembly, and end-of-life stages of the automotive lithium-ion battery life cycle , 2014 .

[13]  Nenad G. Nenadic,et al.  Environmental trade-offs across cascading lithium-ion battery life cycles , 2015, The International Journal of Life Cycle Assessment.

[14]  Mathieux Fabrice,et al.  Feasibility study for setting-up reference values to support the calculation of recyclability / recoverability rates of electr(on)ic products , 2016 .

[15]  Brett Lois,et al.  Putting Science into Standards: Workshop – Summary & Outcomes: Driving Towards Decarbonisation of Transport: Safety, Performance, Second Life and Recycling of Automotive Batteries for e-Vehicles , 2016 .

[16]  Sala Serenella,et al.  The International Reference Life Cycle Data System (ILCD) Handbook - Towards more sustainable production and consumption for a resource-efficient Europe , 2012 .

[17]  Alexis Van Maercke,et al.  EU Methodology for Critical Raw Materials Assessment: Policy Needs and Proposed Solutions for Incremental Improvements , 2017 .

[18]  Markus A. Reuter,et al.  Life cycle impact assessment of the average passenger vehicle in the Netherlands , 2003 .

[19]  Troy R. Hawkins,et al.  Comparative Environmental Life Cycle Assessment of Conventional and Electric Vehicles , 2013 .

[20]  Alessandro Ciocia,et al.  Optimal Power Sharing between Photovoltaic Generators, Wind Turbines, Storage and Grid to Feed Tertiary Sector Users , 2017 .

[21]  Sandia Report,et al.  Energy Storage for the Electricity Grid: Benefits and Market Potential Assessment Guide A Study for the DOE Energy Storage Systems Program , 2010 .

[22]  Herbert White,et al.  End-of-life vehicles , 2014 .

[23]  Joeri Van Mierlo,et al.  Environmental impacts of hybrid, plug-in hybrid, and battery electric vehicles—what can we learn from life cycle assessment? , 2014, The International Journal of Life Cycle Assessment.

[24]  Brett Lois,et al.  Lithium ion battery value chain and related opportunities for Europe , 2016 .

[25]  Daniel Nilsson,et al.  Photovoltaic self-consumption in buildings : A review , 2015 .

[26]  Reinout Heijungs,et al.  Identifying best existing practice for characterization modeling in life cycle impact assessment , 2012, The International Journal of Life Cycle Assessment.

[27]  Rana Pant,et al.  Allocation solutions for secondary material production and end of life recovery: Proposals for product policy initiatives , 2014 .

[28]  Pedro Rodríguez,et al.  Second life battery energy storage system for residential demand response service , 2015, 2015 IEEE International Conference on Industrial Technology (ICIT).

[29]  P. Mokhtarian,et al.  Do changes in neighborhood characteristics lead to changes in travel behavior? A structural equations modeling approach , 2007 .

[30]  Robert Reinhardt,et al.  Critical evaluation of European Union legislation on the second use of degraded traction batteries , 2016, 2016 13th International Conference on the European Energy Market (EEM).

[31]  Manuel Baumann,et al.  The environmental impact of Li-Ion batteries and the role of key parameters – A review , 2017 .

[32]  J. Prins Directive 2003/98/EC of the European Parliament and of the Council , 2006 .

[33]  Marmier Alain,et al.  Assessment of potential bottlenecks along the materials supply chain for the future deployment of low-carbon energy and transport technologies in the EU: Wind power, photovoltaic and electric vehicles technologies, time frame: 2015-2030 , 2016 .

[34]  Serenella Sala,et al.  Natural biotic resources in LCA: Towards an impact assessment model for sustainable supply chain management , 2018, Journal of cleaner production.

[35]  Callie W. Babbitt,et al.  Eco‐Efficiency Analysis of a Lithium‐Ion Battery Waste Hierarchy Inspired by Circular Economy , 2017 .

[36]  Rana Pant,et al.  Rethinking the area of protection "natural resources" in life cycle assessment. , 2015, Environmental science & technology.

[37]  Steven B. Young,et al.  Environmental feasibility of re-use of electric vehicle batteries , 2014 .

[38]  Jae Wan Park,et al.  Off-grid photovoltaic vehicle charge using second life lithium batteries: An experimental and numerical investigation , 2013 .

[39]  John Lippert,et al.  Technical and Economic Feasibility of Applying Used EV Batteries in Stationary Applications , 2003 .

[40]  Fulvio Ardente,et al.  Rationales for and limitations of preferred solutions for multi-functionality problems in LCA: is increased consistency possible? , 2014, The International Journal of Life Cycle Assessment.

[41]  Steffen Görtz,et al.  Battery energy storage for intermittent renewable electricity production : A review and demonstration of energy storage applications permitting higher penetration of renewables , 2015 .

[42]  Thomas Vogt,et al.  Comparative life cycle assessment of battery storage systems for stationary applications. , 2015, Environmental science & technology.

[43]  Hans-Jörg Althaus,et al.  The environmental performance of current and future passenger vehicles: Life cycle assessment based on a novel scenario analysis framework , 2015 .

[44]  Steve Evans,et al.  Business Models for Sustainability: The Case of Second-life Electric Vehicle Batteries , 2016 .

[45]  Paul A. Ardis,et al.  Estimation of State-of-Charge and Capacity of Used Lithium-Ion Cells , 2021 .

[46]  Stefan Spinler,et al.  Valuation of electric vehicle batteries in vehicle-to-grid and battery-to-grid systems , 2012 .

[47]  Michael Hinterstocker,et al.  Increasing residential self-consumption of PV energy by DSM , 2017 .

[48]  James Marco,et al.  Management of intellectual property uncertainty in a remanufacturing strategy for automotive energy storage systems , 2016, Journal of Remanufacturing.

[49]  Kirti Richa,et al.  Sustainable management of lithium-ion batteries after use in electric vehicles , 2016 .

[50]  Callie W. Babbitt,et al.  Economies of scale for future lithium-ion battery recycling infrastructure , 2014 .

[51]  Rana Pant,et al.  Comparing the European Commission product environmental footprint method with other environmental accounting methods , 2015, The International Journal of Life Cycle Assessment.

[52]  D. O M I N I,et al.  Contribution of Li-Ion Batteries to the Environmental Impact of Electric Vehicles , 2010 .

[53]  Robert Reinhardt,et al.  Macro environmental analysis of the electric vehicle battery second use market , 2017, 2017 14th International Conference on the European Energy Market (EEM).

[54]  Roger Sathre,et al.  Energy and climate effects of second-life use of electric vehicle batteries in California through 2050 , 2015 .

[55]  Fulvio Ardente,et al.  Accounting for the environmental benefits of remanufactured products: Method and application , 2018, Journal of cleaner production.

[56]  ThE CirCUlAr,et al.  EU Action Plan for the Circular Economy , 2016 .

[57]  H. Ossenbrink,et al.  DEPLOYMENT PATHWAYS FOR PHOTOVOLTAICS IN THE EU TOWARDS 2020: COMPARING ECONOMIC FACTORS WITH POLICIES AT MUNICIPAL LEVEL , 2015 .

[58]  Joeri Van Mierlo,et al.  A Range-Based Vehicle Life Cycle Assessment Incorporating Variability in the Environmental Assessment of Different Vehicle Technologies and Fuels , 2014 .

[59]  Jeremy Neubauer,et al.  The ability of battery second use strategies to impact plug-in electric vehicle prices and serve uti , 2011 .

[60]  Rana Pant,et al.  Research Needs and Challenges from Science to Decision Support. Lesson Learnt from the Development of the International Reference Life Cycle Data System (ILCD) Recommendations for Life Cycle Impact Assessment , 2012 .

[61]  Anibal T. de Almeida,et al.  Primary and secondary use of electric mobility batteries from a life cycle perspective , 2014 .

[62]  Yan Wang,et al.  Repurposing Used Electric Car Batteries: A Review of Options , 2017 .

[63]  Jeremy Neubauer,et al.  Identifying and Overcoming Critical Barriers to Widespread Second Use of PEV Batteries , 2015 .

[64]  Anders Hammer Strømman,et al.  Life cycle environmental assessment of lithium-ion and nickel metal hydride batteries for plug-in hybrid and battery electric vehicles. , 2011, Environmental science & technology.

[65]  Volker Quaschning,et al.  Sizing of Residential PV Battery Systems , 2014 .